GSTDTAP  > 地球科学
DOI10.5194/acp-18-8373-2018
Maximizing ozone signals among chemical, meteorological, and climatological variability
Brown-Steiner, Benjamin1,2; Selin, Noelle E.2,4,5; Prinn, Ronald G.1,2,5; Monier, Erwan1,2; Tilmes, Simone6; Emmons, Louisa6; Garcia-Menendez, Fernando3
2018-06-15
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2018
卷号18期号:11页码:8373-8388
文章类型Article
语种英语
国家USA
英文摘要

The detection of meteorological, chemical, or other signals in modeled or observed air quality data - such as an estimate of a temporal trend in surface ozone data, or an estimate of the mean ozone of a particular region during a particular season - is a critical component of modern atmospheric chemistry. However, the magnitude of a surface air quality signal is generally small compared to the magnitude of the underlying chemical, meteorological, and climatological variabilities (and their interactions) that exist both in space and in time, and which include variability in emissions and surface processes. This can present difficulties for both policymakers and researchers as they attempt to identify the influence or signal of climate trends (e.g., any pauses in warming trends), the impact of enacted emission reductions policies (e.g., United States NOx State Implementation Plans), or an estimate of the mean state of highly variable data (e. g., summertime ozone over the northeastern United States). Here we examine the scale dependence of the variability of simulated and observed surface ozone data within the United States and the likelihood that a particular choice of temporal or spatial averaging scales produce a misleading estimate of a particular ozone signal. Our main objective is to develop strategies that reduce the likelihood of overconfidence in simulated ozone estimates. We find that while increasing the extent of both temporal and spatial averaging can enhance signal detection capabilities by reducing the noise from variability, a strategic combination of particular temporal and spatial averaging scales can maximize signal detection capabilities over much of the continental US. For signals that are large compared to the meteorological variability (e.g., strong emissions reductions), shorter averaging periods and smaller spatial averaging regions may be sufficient, but for many signals that are smaller than or comparable in magnitude to the underlying meteorological variability, we recommend temporal averaging of 10-15 years combined with some level of spatial averaging (up to several hundred kilometers). If this level of averaging is not practical (e.g., the signal being examined is at a local scale), we recommend some exploration of the spatial and temporal variability to provide context and confidence in the robustness of the result. These results are consistent between simulated and observed data, as well as within a single model with different sets of parameters. The strategies selected in this study are not limited to surface ozone data and could potentially maximize signal detection capabilities within a broad array of climate and chemical observations or model output.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000435406800001
WOS关键词SURFACE OZONE ; ATMOSPHERIC CHEMISTRY ; CLIMATE-CHANGE ; TROPOSPHERIC OZONE ; AIR-QUALITY ; MODEL ; US ; TEMPERATURE ; PROJECTIONS ; EMISSIONS
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/16191
专题地球科学
作者单位1.MIT, Ctr Global Change Sci, 77 Massachusetts Ave, Cambridge, MA 02139 USA;
2.MIT, Joint Program Sci & Policy Global Change, 77 Massachusetts Ave, Cambridge, MA 02139 USA;
3.North Carolina State Univ, Dept Civil Construct & Environm Engn, Raleigh, NC 27695 USA;
4.MIT, Inst Data Syst & Soc, 77 Massachusetts Ave, Cambridge, MA 02139 USA;
5.MIT, Dept Earth Atmospher & Planetary Sci, 77 Massachusetts Ave, Cambridge, MA 02139 USA;
6.Natl Ctr Atmospher Res, Atmospher Chem Observ & Modeling Lab, 3450 Mitchell Lane, Boulder, CO 80301 USA
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Brown-Steiner, Benjamin,Selin, Noelle E.,Prinn, Ronald G.,et al. Maximizing ozone signals among chemical, meteorological, and climatological variability[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(11):8373-8388.
APA Brown-Steiner, Benjamin.,Selin, Noelle E..,Prinn, Ronald G..,Monier, Erwan.,Tilmes, Simone.,...&Garcia-Menendez, Fernando.(2018).Maximizing ozone signals among chemical, meteorological, and climatological variability.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(11),8373-8388.
MLA Brown-Steiner, Benjamin,et al."Maximizing ozone signals among chemical, meteorological, and climatological variability".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.11(2018):8373-8388.
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