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DOI10.1029/2019WR025021
Field Comparison of DNA-Labeled Nanoparticle and Solute Tracer Transport in a Fractured Crystalline Rock
Kittilae, A.1; Jalali, M. R.2,3; Evans, K. F.1; Willmann, M.4,5; Saar, M. O.1; Kong, X. -Z.1
2019-08-01
发表期刊WATER RESOURCES RESEARCH
ISSN0043-1397
EISSN1944-7973
出版年2019
卷号55期号:8页码:6577-6595
文章类型Article
语种英语
国家Switzerland; Germany
英文摘要

Field tracer experiments were conducted to examine tracer transport properties in a fracture-dominated crystalline rock mass at the Grimsel Test Site, Switzerland. In the experiments reported here, both the DNA nanotracers and solute dye tracers were simultaneously injected. We compare the transport of DNA nanotracers to solute dye tracers by performing temporal moment analysis on the recorded tracer breakthrough curves and estimate the swept volumes and flow geometries. The DNA nanotracers, approximately 166 nm in diameter, are observed to travel at a higher average velocity than the solutes but with lower mass recoveries, lower swept volumes, and less dispersion. Moreover, size exclusion and potentially, particle density effects are observed during the transport of the DNA nanotracers. Compared to solute tracers, the greatest strength of DNA nanotracers is the demonstrated zero signal interference of background noise during repeat or multitracer tests. This work provides encouraging results in advancing the use of DNA nanotracers in hydrogeological applications, for example, during contaminant transport investigations or geothermal reservoir characterization.


领域资源环境
收录类别SCI-E
WOS记录号WOS:000490973700013
WOS关键词POLYDISPERSE COLLOID TRANSPORT ; MASS-TRANSFER ; RADIONUCLIDE TRANSPORT ; MIGRATION EXPERIMENTS ; MATRIX DIFFUSION ; FLOW ; TESTS ; AQUIFER ; SOIL ; PERMEABILITY
WOS类目Environmental Sciences ; Limnology ; Water Resources
WOS研究方向Environmental Sciences & Ecology ; Marine & Freshwater Biology ; Water Resources
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/185853
专题资源环境科学
作者单位1.Swiss Fed Inst Technol, Inst Geophys, Geothermal Energy & Geofluids Grp, Zurich, Switzerland;
2.Swiss Fed Inst Technol, SCCER SoE, Zurich, Switzerland;
3.Rhein Westfal TH Aachen, Dept Engn Geol & Hydrogeol, Aachen, Germany;
4.Swiss Fed Inst Technol, Inst Environm Engn, Zurich, Switzerland;
5.Solexperts AG, Moenchaltorf, Switzerland
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Kittilae, A.,Jalali, M. R.,Evans, K. F.,et al. Field Comparison of DNA-Labeled Nanoparticle and Solute Tracer Transport in a Fractured Crystalline Rock[J]. WATER RESOURCES RESEARCH,2019,55(8):6577-6595.
APA Kittilae, A.,Jalali, M. R.,Evans, K. F.,Willmann, M.,Saar, M. O.,&Kong, X. -Z..(2019).Field Comparison of DNA-Labeled Nanoparticle and Solute Tracer Transport in a Fractured Crystalline Rock.WATER RESOURCES RESEARCH,55(8),6577-6595.
MLA Kittilae, A.,et al."Field Comparison of DNA-Labeled Nanoparticle and Solute Tracer Transport in a Fractured Crystalline Rock".WATER RESOURCES RESEARCH 55.8(2019):6577-6595.
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