Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.5194/acp-19-11013-2019 |
Arabitol, mannitol, and glucose as tracers of primary biogenic organic aerosol: the influence of environmental factors on ambient air concentrations and spatial distribution over France | |
Samake, Abdoulaye1; Jaffrezo, Jean-Luc1; Favez, Olivier2,3; Weber, Samuel1; Jacob, Veronique1; Canete, Trishalee1; Albinet, Alexandre2,3; Charron, Aurelie1,4; Riffault, Veronique5; Perdrix, Esperanza5; Waked, Antoine1; Golly, Benjamin1; Salameh, Dalia1,18; Chevrier, Florie1,6,13; Oliveira, Diogo Miguel2,5; Besombes, Jean-Luc6; Martins, Jean M. F.1; Bonnaire, Nicolas7; Conil, Sebastien8; Guillaud, Geraldine9; Mesbah, Boualem10; Rocq, Benoit11; Robic, Pierre-Yves12; Hulin, Agnes13; Le Meur, Sebastien14; Descheemaecker, Maxence15; Chretien, Eve16; Marchand, Nicolas17; Uzu, Gaelle1 | |
2019-08-29 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS
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ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2019 |
卷号 | 19期号:16页码:11013-11030 |
文章类型 | Article |
语种 | 英语 |
国家 | France |
英文摘要 | The primary sugar compounds (SCs, defined as glucose, arabitol, and mannitol) are widely recognized as suitable molecular markers to characterize and apportion primary biogenic organic aerosol emission sources. This work improves our understanding of the spatial behavior and distribution of these chemical species and evidences their major effective environmental drivers. We conducted a large study focusing on the daily (24 h) PM10 SC concentrations for 16 increasing space scale sites (local to nationwide), over at least 1 complete year. These sites are distributed in several French geographic areas of different environmental conditions. Our analyses, mainly based on the examination of the short-term evolutions of SC concentrations, clearly show distance-dependent correlations. SC concentration evolutions are highly synchronous at an urban city scale and remain well correlated throughout the same geographic regions, even if the sites are situated in different cities. However, sampling sites located in two distinct geographic areas are poorly correlated. Such a pattern indicates that the processes responsible for the evolution of the atmospheric SC concentrations present a spatial homogeneity over typical areas of at least tens of kilometers. Local phenomena, such as the resuspension of topsoil and associated microbiota, do no account for the major emissions processes of SC in urban areas not directly influenced by agricultural activities. The concentrations of SC and cellulose display remarkably synchronous temporal evolution cycles at an urban site in Grenoble, indicating a common source ascribed to vegetation. Additionally, higher concentrations of SC at another site located in a crop field region occur during each harvest periods, indicating resuspension processes of plant materials (crop detritus, leaf debris) and associated microbiota for agricultural and nearby urbanized areas. Finally, ambient air temperature, relative humidity, and vegetation density constitute the main effective drivers of SC atmospheric concentrations. |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000483093000006 |
WOS关键词 | WESTERN NORTH PACIFIC ; LONG-RANGE TRANSPORT ; SOURCE APPORTIONMENT ; SEASONAL-VARIATIONS ; ATMOSPHERIC BIOAEROSOL ; CARBONACEOUS AEROSOLS ; PARTICULATE MATTER ; MARKER COMPOUNDS ; SUGAR-ALCOHOLS ; FUNGAL SPORES |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/186295 |
专题 | 地球科学 |
作者单位 | 1.Univ Grenoble Alpes, INP G, CNRS, IRD,IGE UMR 5001, F-38000 Grenoble, France; 2.INERIS, Parc Technol Alata,BP 2, F-60550 Verneuil En Halatte, France; 3.LCSQA, F-60550 Verneuil En Halatte, France; 4.IFSTTAR, F-69675 Bron, France; 5.Univ Lille, IMT Lille Douai, SAGE Dept Sci Atmosphere & Genie Environm, F-59000 Lille, France; 6.Univ Savoie Mt Blanc, LCME, F-73000 Chambery, France; 7.UMR CNRS CEA UVSQ, LSCE, F-91191 Gif Sur Yvette, France; 8.ANDRA DRD GES Observ Perenne Environm, F-55290 Bure, France; 9.Atmo Auvergne Rhone Alpes, F-38400 Grenoble, France; 10.Air PACA, F-13294 Marseille, France; 11.Atmo Hauts France, F-59000 Lille, France; 12.Atmo Occitanie, F-31330 Toulouse, France; 13.Atmo Nouvelle Aquitaine, F-33000 Bordeaux, France; 14.Atmo Normandie, F-76000 Rouen, France; 15.Lig Air, F-45590 St Cyr En Val, France; 16.Atmo Grand Est, F-16034 Strasbourg, France; 17.Univ Aix Marseille, LCE UMR7376, F-13331 Marseille, France; 18.Airport Pollut Control Author ACNUSA, F-75007 Paris, France |
推荐引用方式 GB/T 7714 | Samake, Abdoulaye,Jaffrezo, Jean-Luc,Favez, Olivier,et al. Arabitol, mannitol, and glucose as tracers of primary biogenic organic aerosol: the influence of environmental factors on ambient air concentrations and spatial distribution over France[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019,19(16):11013-11030. |
APA | Samake, Abdoulaye.,Jaffrezo, Jean-Luc.,Favez, Olivier.,Weber, Samuel.,Jacob, Veronique.,...&Uzu, Gaelle.(2019).Arabitol, mannitol, and glucose as tracers of primary biogenic organic aerosol: the influence of environmental factors on ambient air concentrations and spatial distribution over France.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(16),11013-11030. |
MLA | Samake, Abdoulaye,et al."Arabitol, mannitol, and glucose as tracers of primary biogenic organic aerosol: the influence of environmental factors on ambient air concentrations and spatial distribution over France".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.16(2019):11013-11030. |
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