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DOI10.1073/pnas.1808101115
Insights into the origin of carbonaceous chondrite organics from their triple oxygen isotope composition
Tartese, Romain1; Chaussidon, Marc2; Gurenko, Andrey3; Delarue, Frederic4; Robert, Francois5,6
2018-08-21
发表期刊PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
ISSN0027-8424
出版年2018
卷号115期号:34页码:8535-8540
文章类型Article
语种英语
国家England; France
英文摘要

Dust grains of organic matter were the main reservoir of C and N in the forming Solar System and are thus considered to be an essential ingredient for the emergence of life. However, the physical environment and the chemical mechanisms at the origin of these organic grains are still highly debated. In this study, we report high-precision triple oxygen isotope composition for insoluble organic matter isolated from three emblematic carbonaceous chondrites, Orgueil, Murchison, and Cold Bokkeveld. These results suggest that the O isotope composition of carbonaceous chondrite insoluble organic matter falls on a slope 1 correlation line in the triple oxygen isotope diagram. The lack of detectable mass-dependent O isotopic fractionation, indicated by the slope 1 line, suggests that the bulk of carbonaceous chondrite organics did not form on asteroidal parent bodies during low-temperature hydrothermal events. On the other hand, these O isotope data, together with the H and N isotope characteristics of insoluble organic matter, may indicate that parent bodies of different carbonaceous chondrite types largely accreted organics formed locally in the protosolar nebula, possibly by photochemical dissociation of C-rich precursors.


英文关键词carbonaceous chondrites organic matter oxygen isotopes protosolar nebula secondary ion mass spectrometry
领域地球科学 ; 气候变化 ; 资源环境
收录类别SCI-E
WOS记录号WOS:000442351000043
WOS关键词MOLECULAR-STRUCTURE ; ORGUEIL METEORITE ; GAS-PHASE ; MATTER ; MURCHISON ; ALLENDE ; DEUTERIUM ; HYDROGEN ; FRACTIONATION ; HETEROGENEITY
WOS类目Multidisciplinary Sciences
WOS研究方向Science & Technology - Other Topics
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文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/204969
专题地球科学
资源环境科学
气候变化
作者单位1.Univ Manchester, Sch Earth & Environm Sci, Manchester M13 9PL, Lancs, England;
2.Univ Paris Diderot, CNRS UMR 7154, Inst Phys Globe Paris, Univ Sorbonne Paris Cite, F-75238 Paris, France;
3.Univ Lorraine, Ctr Recherches Petrog & Geochim, UMR 7358, F-54501 Vandoeuvre Les Nancy, France;
4.Univ Paris 06, Sorbonne Univ, CNRS, Ecole Prat Hautes Etud,Paris Sci & Lettres,UMR Mi, Paris, France;
5.Univ Paris 06, Museum Natl Hist Nat, Sorbonne Univ, Inst Mineral Phys Mat & Cosmochim,CNRS, F-75005 Paris, France;
6.Inst Rech Dev, F-75005 Paris, France
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GB/T 7714
Tartese, Romain,Chaussidon, Marc,Gurenko, Andrey,et al. Insights into the origin of carbonaceous chondrite organics from their triple oxygen isotope composition[J]. PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,2018,115(34):8535-8540.
APA Tartese, Romain,Chaussidon, Marc,Gurenko, Andrey,Delarue, Frederic,&Robert, Francois.(2018).Insights into the origin of carbonaceous chondrite organics from their triple oxygen isotope composition.PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,115(34),8535-8540.
MLA Tartese, Romain,et al."Insights into the origin of carbonaceous chondrite organics from their triple oxygen isotope composition".PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA 115.34(2018):8535-8540.
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