GSTDTAP  > 地球科学
DOI10.1073/pnas.1804250115
Current CaCO3 dissolution at the seafloor caused by anthropogenic CO2
Sulpis, Olivier1,2; Boudreau, Bernard P.3; Mucci, Alfonso1,2; Jenkins, Chris4; Trossman, David S.5; Arbic, Brian K.6; Key, Robert M.7
2018-11-13
发表期刊PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
ISSN0027-8424
出版年2018
卷号115期号:46页码:11700-11705
文章类型Article
语种英语
国家Canada; USA
英文摘要

Oceanic uptake of anthropogenic CO2 leads to decreased pH, carbonate ion concentration, and saturation state with respect to CaCO3 minerals, causing increased dissolution of these minerals at the deep seafloor. This additional dissolution will figure prominently in the neutralization of man-made CO2 . However, there has been no concerted assessment of the current extent of anthropogenic CaCO3 dissolution at the deep seafloor. Here, recent databases of bottom-water chemistry, benthic currents, and CaCO3 content of deep-sea sediments are combined with a rate model to derive the global distribution of benthic calcite dissolution rates and obtain primary confirmation of an anthropogenic component. By comparing preindustrial with present-day rates, we determine that significant anthropogenic dissolution now occurs in the western North Atlantic, amounting to 40-100% of the total seafloor dissolution at its most intense locations. At these locations, the calcite compensation depth has risen similar to 300 m. Increased benthic dissolution was also revealed at various hot spots in the southern extent of the Atlantic, Indian, and Pacific Oceans. Our findings place constraints on future predictions of ocean acidification, are consequential to the fate of benthic calcifiers, and indicate that a by-product of human activities is currently altering the geological record of the deep sea.


英文关键词ocean acidification seafloor CaCO3 dissolution anthropogenic CO2
领域地球科学 ; 气候变化 ; 资源环境
收录类别SCI-E
WOS记录号WOS:000449934400033
WOS关键词TURBULENT MASS-TRANSFER ; FOSSIL-FUEL CO2 ; OCEAN ACIDIFICATION ; DIFFUSIVE SUBLAYER ; GLOBAL OCEAN ; WATER ; CARBON ; MODEL ; SATURATION ; CALCITE
WOS类目Multidisciplinary Sciences
WOS研究方向Science & Technology - Other Topics
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文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/205011
专题地球科学
资源环境科学
气候变化
作者单位1.McGill Univ, GEOTOP, Montreal, PQ H3A 0E8, Canada;
2.McGill Univ, Dept Earth & Planetary Sci, Montreal, PQ H3A 0E8, Canada;
3.Dalhousie Univ, Dept Oceanog, Halifax, NS B3H 4R2, Canada;
4.Univ Colorado, Inst Arctic & Alpine Res, Boulder, CO 80309 USA;
5.Univ Texas Austin, Inst Computat Engn & Sci, Austin, TX 78712 USA;
6.Univ Michigan, Dept Earth & Environm Sci, Ann Arbor, MI 48109 USA;
7.Princeton Univ, Atmospher & Ocean Sci, Princeton, NJ 08540 USA
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GB/T 7714
Sulpis, Olivier,Boudreau, Bernard P.,Mucci, Alfonso,et al. Current CaCO3 dissolution at the seafloor caused by anthropogenic CO2[J]. PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,2018,115(46):11700-11705.
APA Sulpis, Olivier.,Boudreau, Bernard P..,Mucci, Alfonso.,Jenkins, Chris.,Trossman, David S..,...&Key, Robert M..(2018).Current CaCO3 dissolution at the seafloor caused by anthropogenic CO2.PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,115(46),11700-11705.
MLA Sulpis, Olivier,et al."Current CaCO3 dissolution at the seafloor caused by anthropogenic CO2".PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA 115.46(2018):11700-11705.
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