Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.5194/acp-18-16793-2018 |
Impacts on cloud radiative effects induced by coexisting aerosols converted from international shipping and maritime DMS emissions | |
Jin, Qinjian1; Grandey, Benjamin S.2; Rothenberg, Daniel1; Avramov, Alexander1,3; Wang, Chien1,2 | |
2018-11-28 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS
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ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2018 |
卷号 | 18期号:22页码:16793-16808 |
文章类型 | Article |
语种 | 英语 |
国家 | USA; Singapore |
英文摘要 | International shipping emissions (ISE), particularly sulfur dioxide, can influence the global radiation budget by interacting with clouds and radiation after being oxidized into sulfate aerosols. A better understanding of the uncertainties in estimating the cloud radiative effects (CREs) of ISE is of great importance in climate science. Many international shipping tracks cover oceans with substantial natural dimethyl sulfide (DMS) emissions. The interplay between these two major aerosol sources on CREs over vast oceanic regions with a relatively low aerosol concentration is an intriguing yet poorly addressed issue confounding estimation of the CREs of ISE. Using an Earth system model including two aerosol modules with different aerosol mixing configurations, we derive a significant global net CRE of ISE (-0.153 W m(-2) with a standard error of +/- 0.004 W m(-2)) when using emissions consistent with current ship emission regulations. This global net CRE would become much weaker and actually insignificant (-0.001 W m(-2) standard error of +/- 0.007 W m(-2)) if a more stringent regulation were adopted. We then reveal that the ISE-induced CRE would achieve a significant enhancement when a lower DMS emission is prescribed in the simulations, owing to the sublinear relationship between aerosol concentration and cloud response. In addition, this study also demonstrates that the representation of certain aerosol processes, such as mixing states, can influence the magnitude and pattern of the ISE-induced CRE. These findings suggest a reevaluation of the ISE-induced CRE with consideration of DMS variability. |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000451399900002 |
WOS关键词 | COMMUNITY ATMOSPHERE MODEL ; SULFATE AEROSOL ; GLOBAL-MODEL ; CLIMATE ; REPRESENTATION ; ACTIVATION ; SENSITIVITY ; HYGROSCOPICITY |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/20570 |
专题 | 地球科学 |
作者单位 | 1.MIT, Ctr Global Change Sci, 77 Massachusetts Ave, Cambridge, MA 02139 USA; 2.Singapore MIT Alliance Res & Technol, Ctr Environm Sensing & Modelling, Singapore, Singapore; 3.Emory Univ, Dept Environm Sci, Atlanta, GA 30322 USA |
推荐引用方式 GB/T 7714 | Jin, Qinjian,Grandey, Benjamin S.,Rothenberg, Daniel,et al. Impacts on cloud radiative effects induced by coexisting aerosols converted from international shipping and maritime DMS emissions[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(22):16793-16808. |
APA | Jin, Qinjian,Grandey, Benjamin S.,Rothenberg, Daniel,Avramov, Alexander,&Wang, Chien.(2018).Impacts on cloud radiative effects induced by coexisting aerosols converted from international shipping and maritime DMS emissions.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(22),16793-16808. |
MLA | Jin, Qinjian,et al."Impacts on cloud radiative effects induced by coexisting aerosols converted from international shipping and maritime DMS emissions".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.22(2018):16793-16808. |
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