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DOI10.5194/acp-18-16793-2018
Impacts on cloud radiative effects induced by coexisting aerosols converted from international shipping and maritime DMS emissions
Jin, Qinjian1; Grandey, Benjamin S.2; Rothenberg, Daniel1; Avramov, Alexander1,3; Wang, Chien1,2
2018-11-28
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2018
卷号18期号:22页码:16793-16808
文章类型Article
语种英语
国家USA; Singapore
英文摘要

International shipping emissions (ISE), particularly sulfur dioxide, can influence the global radiation budget by interacting with clouds and radiation after being oxidized into sulfate aerosols. A better understanding of the uncertainties in estimating the cloud radiative effects (CREs) of ISE is of great importance in climate science. Many international shipping tracks cover oceans with substantial natural dimethyl sulfide (DMS) emissions. The interplay between these two major aerosol sources on CREs over vast oceanic regions with a relatively low aerosol concentration is an intriguing yet poorly addressed issue confounding estimation of the CREs of ISE. Using an Earth system model including two aerosol modules with different aerosol mixing configurations, we derive a significant global net CRE of ISE (-0.153 W m(-2) with a standard error of +/- 0.004 W m(-2)) when using emissions consistent with current ship emission regulations. This global net CRE would become much weaker and actually insignificant (-0.001 W m(-2) standard error of +/- 0.007 W m(-2)) if a more stringent regulation were adopted. We then reveal that the ISE-induced CRE would achieve a significant enhancement when a lower DMS emission is prescribed in the simulations, owing to the sublinear relationship between aerosol concentration and cloud response. In addition, this study also demonstrates that the representation of certain aerosol processes, such as mixing states, can influence the magnitude and pattern of the ISE-induced CRE. These findings suggest a reevaluation of the ISE-induced CRE with consideration of DMS variability.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000451399900002
WOS关键词COMMUNITY ATMOSPHERE MODEL ; SULFATE AEROSOL ; GLOBAL-MODEL ; CLIMATE ; REPRESENTATION ; ACTIVATION ; SENSITIVITY ; HYGROSCOPICITY
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/20570
专题地球科学
作者单位1.MIT, Ctr Global Change Sci, 77 Massachusetts Ave, Cambridge, MA 02139 USA;
2.Singapore MIT Alliance Res & Technol, Ctr Environm Sensing & Modelling, Singapore, Singapore;
3.Emory Univ, Dept Environm Sci, Atlanta, GA 30322 USA
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GB/T 7714
Jin, Qinjian,Grandey, Benjamin S.,Rothenberg, Daniel,et al. Impacts on cloud radiative effects induced by coexisting aerosols converted from international shipping and maritime DMS emissions[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(22):16793-16808.
APA Jin, Qinjian,Grandey, Benjamin S.,Rothenberg, Daniel,Avramov, Alexander,&Wang, Chien.(2018).Impacts on cloud radiative effects induced by coexisting aerosols converted from international shipping and maritime DMS emissions.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(22),16793-16808.
MLA Jin, Qinjian,et al."Impacts on cloud radiative effects induced by coexisting aerosols converted from international shipping and maritime DMS emissions".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.22(2018):16793-16808.
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