Tropospheric Photochemistry of Carbonyls: Elucidation of Quantum Yields to Quantify the Role of Ketones in Production of HOx and PAN-type Compounds in the Atmosphere

GSTDTAP

项目编号	1922619
	Tropospheric Photochemistry of Carbonyls: Elucidation of Quantum Yields to Quantify the Role of Ketones in Production of HOx and PAN-type Compounds in the Atmosphere
	Akkihebbal Ravishankara (Principal Investigator)
主持机构	Colorado State University
项目开始年	2019
	2019-08-01
项目结束日期	2022-07-31
资助机构	US-NSF
项目类别	Standard Grant
项目经费	559175(USD)
国家	美国
语种	英语
英文摘要	This project will use state-of-the-art measurement methods to investigate photolysis reactions that are important in the atmosphere. Specifically, the team will develop a new methodology for quantum yield measurements of complex molecules using chemical ionization mass spectrometry (CIMS). Initial efforts will focus on investigating reactions which arise from radiation interacting with ketones in the upper troposphere. The research team will use the results to better understand the concentrations of reaction species in the upper troposphere. The project will also support training of a graduate study and a postdoctoral researcher. The researchers will use CIMS to detect radical reaction products from the photolysis of acetone and other ketones as a function of wavelength, O2, pressure, and temperature. Data will provide experimental constraints which will contribute to our understanding of the upper tropospheric HOx and PAN budgets. Additionally, this new method for measuring quantum yields has the potentially to be used in numerous future experiments. This award reflects NSF's statutory mission and has been deemed worthy of support through evaluation using the Foundation's intellectual merit and broader impacts review criteria.
文献类型	项目
条目标识符	http://119.78.100.173/C666/handle/2XK7JSWQ/213855
专题	环境与发展全球科技态势
推荐引用方式 GB/T 7714	Akkihebbal Ravishankara .Tropospheric Photochemistry of Carbonyls: Elucidation of Quantum Yields to Quantify the Role of Ketones in Production of HOx and PAN-type Compounds in the Atmosphere.2019.