Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.5194/acp-2020-170 |
Snow heterogeneous reactivity of bromide with ozone lost during snow metamorphism | |
Jacinta Edebeli, Jürg C. Trachsel, Sven E. Avak, Markus Ammann, Martin Schneebeli, Anja Eichler, and Thorsten Bartels-Rausch | |
2020-04-22 | |
发表期刊 | Atmospheric Chemistry and Physics
![]() |
出版年 | 2020 |
英文摘要 | Earth's snow cover is very dynamic on diurnal time scales. The changes to the snow structure during this metamorphism have wide ranging impacts such as on avalanche formation and on the capacity of surface snow to exchange trace gases with the atmosphere. Here, we investigate the influence of dry metamorphism, which involves fluxes of water vapor, on the chemical reactivity of bromide in the snow. For this, the heterogeneous reactive loss of ozone at a concentration of 5–6 x 1012 molecules cm-3 is investigated in artificial, shock-frozen snow samples doped with 6.2 μM sodium bromide and with varying metamorphism history. The oxidation of bromide in snow is one reaction initiating polar bromine releases and ozone depletions. We find that the heterogeneous reactivity of bromide is completely absent from the air-ice interface in snow after 12 days of temperature gradient metamorphism and suggest that burial of non-volatile bromide salts occurs when the snow matrix is restructuring during metamorphism. Impacts on polar atmospheric chemistry are discussed. |
领域 | 地球科学 |
URL | 查看原文 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/248956 |
专题 | 地球科学 |
推荐引用方式 GB/T 7714 | Jacinta Edebeli, Jürg C. Trachsel, Sven E. Avak, Markus Ammann, Martin Schneebeli, Anja Eichler, and Thorsten Bartels-Rausch. Snow heterogeneous reactivity of bromide with ozone lost during snow metamorphism[J]. Atmospheric Chemistry and Physics,2020. |
APA | Jacinta Edebeli, Jürg C. Trachsel, Sven E. Avak, Markus Ammann, Martin Schneebeli, Anja Eichler, and Thorsten Bartels-Rausch.(2020).Snow heterogeneous reactivity of bromide with ozone lost during snow metamorphism.Atmospheric Chemistry and Physics. |
MLA | Jacinta Edebeli, Jürg C. Trachsel, Sven E. Avak, Markus Ammann, Martin Schneebeli, Anja Eichler, and Thorsten Bartels-Rausch."Snow heterogeneous reactivity of bromide with ozone lost during snow metamorphism".Atmospheric Chemistry and Physics (2020). |
条目包含的文件 | 条目无相关文件。 |
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。
修改评论