GSTDTAP  > 地球科学
DOI10.5194/acp-2020-399
The impact of urban land-surface on extreme air pollution over central Europe
Peter Huszar, Jan Karlický, Jana Ďoubalová, Tereza Nováková, Kateřina Šindelářová, Filip Švábik, Michal Belda, Tomáš Halenka, and Michal Žák
2020-06-24
发表期刊Atmospheric Chemistry and Physics
出版年2020
英文摘要This paper deals with the urban land-surface impact (i.e. the urban canopy meteorological forcing; UCMF) on extreme air pollution for selected central European cities for present-day climate conditions (2015–2016) using three regional climate-chemistry models: the regional climate models RegCM and WRF-Chem (its meteorological part), the chemistry transport model CAMx coupled to either RegCM and WRF and the chemical component of WRF-Chem. Most of the studies focused on the change of average conditions or only on a selected winter and summer air pollution episode. Here we extend these studies by focusing on long term extreme air pollution levels by looking at not only the change of average values but also their high (and low) percentile values and we combine the analysis with investigating selected high pollution episodes too. As extreme air pollution is often linked to extreme values of meteorological variables (e.g. low planetary boundary layer height, low winds, high temperatures), the extreme meteorological modifications will be analyzed too. The validation of model results shows reasonable model performance for regional scale temperature and precipitation. Ozone is overestimated by about 10–20 μg m−3, on the other hand, extreme summertime ozone values are underestimated by all models. Modeled nitrogen dioxide (NO2) concentrations are well correlated with observations, but results are marked with a systematic underestimation up to 20 μg m−3. PM2.5 (particles with diameter < 2.5 μg m−3) are systematically underestimated in most of the models by around 5 μg m−3.

Our results show that the impact on extreme values of meteorological variables can be substantially different from that of the impact on average ones: low (5 % percentile) temperature in winter responds to UCMF much more than average values, while in summer, 95 % percentiles increase more than averages. The impact on boundary layer height (PBLH), i.e. its increase is stronger for thicker PBLs and wind-speed is reduced much more for strong winds compared to average ones. The modeled changes of ozone (O3), NO2 and PM2.5 show the expected pattern, i.e. increase in average 8-hour O3 up to 2–3 ppbv, decrease of daily average NO2 by around 2–4 ppbv and decrease of daily average PM2.5 by around −2 μg m−3. Regarding the impact on extreme (95 % percentile) values of these pollutants, the impact on ozone at the high-end of the distribution is rather similar to the impact on average 8-hour values. A different picture is obtained however for extreme values of NO2 and PM2.5. The impact on the 95 % values is almost 2 times larger than the impact on the daily averages for both pollutants. The simulated impact on extreme values further well corresponds to the UCMF impact simulated for the selected high pollution episodes. Our results bring light to the principal question: whether extreme air quality is modified by urban land-surface with a different magnitude compared to the impact on average air pollution. We showed that this is indeed true for NO2 and PM2.5 while in case of ozone, our results did not show substantial differences between the impact on mean and extreme values.

领域地球科学
URL查看原文
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/278079
专题地球科学
推荐引用方式
GB/T 7714
Peter Huszar, Jan Karlický, Jana Ďoubalová, Tereza Nováková, Kateřina Šindelářová, Filip Švábik, Michal Belda, Tomáš Halenka, and Michal Žák. The impact of urban land-surface on extreme air pollution over central Europe[J]. Atmospheric Chemistry and Physics,2020.
APA Peter Huszar, Jan Karlický, Jana Ďoubalová, Tereza Nováková, Kateřina Šindelářová, Filip Švábik, Michal Belda, Tomáš Halenka, and Michal Žák.(2020).The impact of urban land-surface on extreme air pollution over central Europe.Atmospheric Chemistry and Physics.
MLA Peter Huszar, Jan Karlický, Jana Ďoubalová, Tereza Nováková, Kateřina Šindelářová, Filip Švábik, Michal Belda, Tomáš Halenka, and Michal Žák."The impact of urban land-surface on extreme air pollution over central Europe".Atmospheric Chemistry and Physics (2020).
条目包含的文件
条目无相关文件。
个性服务
推荐该条目
保存到收藏夹
查看访问统计
导出为Endnote文件
谷歌学术
谷歌学术中相似的文章
[Peter Huszar, Jan Karlický, Jana Ďoubalová, Tereza Nováková, Kateřina Šindelářová, Filip Švábik, Michal Belda, Tomáš Halenka, and Michal Žák]的文章
百度学术
百度学术中相似的文章
[Peter Huszar, Jan Karlický, Jana Ďoubalová, Tereza Nováková, Kateřina Šindelářová, Filip Švábik, Michal Belda, Tomáš Halenka, and Michal Žák]的文章
必应学术
必应学术中相似的文章
[Peter Huszar, Jan Karlický, Jana Ďoubalová, Tereza Nováková, Kateřina Šindelářová, Filip Švábik, Michal Belda, Tomáš Halenka, and Michal Žák]的文章
相关权益政策
暂无数据
收藏/分享
所有评论 (0)
暂无评论
 

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。