GSTDTAP  > 地球科学
DOI10.5194/acp-20-203-2020
Local and synoptic meteorological influences on daily variability in summertime surface ozone in eastern China
Han, Han1; Liu, Jane1,2; Shu, Lei1; Wang, Tijian1; Yuan, Huiling1
2020-01-06
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2020
卷号20期号:1页码:203-222
文章类型Article
语种英语
国家Peoples R China; Canada
英文摘要

Ozone pollution in China is influenced by meteorological processes on multiple scales. Using regression analysis and weather classification, we statistically assess the impacts of local and synoptic meteorology on daily variability in surface ozone in eastern China in summer during 2013-2018. In this period, summertime surface ozone in eastern China (20-42 degrees N, 110-130 degrees E) is among the highest in the world, with regional means of 73.1 and 114.7 mu g m(-3), respectively, in daily mean and daily maximum 8 h average. Through developing a multiple linear regression (MLR) model driven by local and synoptic weather factors, we establish a quantitative linkage between the daily mean ozone concentrations and meteorology in the study region. The meteorology described by the MLR can explain similar to 43 % of the daily variability in summertime surface ozone across eastern China. Among local meteorological factors, relative humidity is the most influential variable in the center and south of eastern China, including the Yangtze River Delta and the Pearl River Delta regions, while temperature is the most influential variable in the north, covering the Beijing-Tianjin-Hebei region. To further examine the synoptic influence of weather conditions explicitly, six predominant synoptic weather patterns (SWPs) over eastern China in summer are objectively identified using the self-organizing map clustering technique. The six SWPs are formed under the integral influence of the East Asian summer monsoon, the western Pacific subtropical high, the Meiyu front, and the typhoon activities. On average, regionally, two SWPs bring about positive ozone anomalies (1.1 mu g m(-3) or 1.7 % and 2.7 mu g m(-3) or 4.6 %), when eastern China is under a weak cyclone system or under the prevailing southerly wind. The impact of SWPs on the daily variability in surface ozone varies largely within eastern China. The maximum impact can reach +/- 8 mu g m(-3) or +/- 16 % of the daily mean in some areas. A combination of the regression and the clustering approaches suggests a strong performance of the MLR in predicting the sensitivity of surface ozone in eastern China to the variation of synoptic weather. Our assessment highlights the importance of meteorology in modulating ozone pollution over China.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000505953600002
WOS关键词YANGTZE-RIVER DELTA ; PARTICULATE MATTER PM2.5 ; AIR-QUALITY ; TROPOSPHERIC OZONE ; BOUNDARY-LAYER ; WEATHER PATTERNS ; UNITED-STATES ; HONG-KONG ; INTERCONTINENTAL TRANSPORT ; ANTHROPOGENIC EMISSIONS
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/278538
专题地球科学
作者单位1.Nanjing Univ, Sch Atmospher Sci, Nanjing, Jiangsu, Peoples R China;
2.Univ Toronto, Dept Geog & Planning, Toronto, ON, Canada
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GB/T 7714
Han, Han,Liu, Jane,Shu, Lei,et al. Local and synoptic meteorological influences on daily variability in summertime surface ozone in eastern China[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2020,20(1):203-222.
APA Han, Han,Liu, Jane,Shu, Lei,Wang, Tijian,&Yuan, Huiling.(2020).Local and synoptic meteorological influences on daily variability in summertime surface ozone in eastern China.ATMOSPHERIC CHEMISTRY AND PHYSICS,20(1),203-222.
MLA Han, Han,et al."Local and synoptic meteorological influences on daily variability in summertime surface ozone in eastern China".ATMOSPHERIC CHEMISTRY AND PHYSICS 20.1(2020):203-222.
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