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DOI | 10.5194/acp-20-4209-2020 |
Influence of the dry aerosol particle size distribution and morphology on the cloud condensation nuclei activation. An experimental and theoretical investigation | |
Wu, Junteng1; Faccinetto, Alessandro1; Grimonprez, Symphorien1; Batut, Sebastien1; Yon, Jerome2; Desgroux, Pascale1; Petitprez, Denis1 | |
2020-04-08 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS |
ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2020 |
卷号 | 20期号:7页码:4209-4225 |
文章类型 | Article |
语种 | 英语 |
国家 | France |
英文摘要 | Combustion and other high-temperature processes frequently result in the emission of aerosols in the form of polydisperse fractal-like aggregates made of condensedphase nanoparticles (soot for instance). If certain conditions are met, the emitted aerosol particles are known to evolve into important cloud condensation nuclei (CCN) in the atmosphere. In this work, the hygroscopic parameter kappa of complex morphology aggregates is calculated from the supersaturation-dependent activated fraction F-a = F-a(SS) in the frame of kappa-Kohler theory. The particle size distribution is approximated with the morphology-corrected volume equivalent diameter calculated from the electrical mobility diameter by taking into account the diameter of the primary particle and the fractal dimension of the aggregate experimentally obtained from transmission electron microscopy measurements. Activation experiments are performed in water supersaturation conditions using a commercial CCN-100 condensation nuclei counter. The model is tested in closeto-ideal conditions of size-selected, isolated spherical particles (ammonium sulfate nanoparticles dispersed in nitrogen), then with complex polydisperse fractal-like aggregates (soot particles activated by exposure to ozone with kappa as low as 5 x 10(-5)) that represent realistic anthropogenic emissions in the atmosphere. |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000525365900002 |
WOS关键词 | SOOT PARTICLES ; HYGROSCOPIC GROWTH ; STRUCTURAL-ANALYSIS ; CCN ACTIVATION ; MIXING STATE ; NUCLEATION ; FLAMES ; NANOSTRUCTURE ; OXIDATION ; MODEL |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/278740 |
专题 | 地球科学 |
作者单位 | 1.Lille Univ, CNRS PC2A, F-59000 Lille, France; 2.Normandie Univ, CNRS CORIA, INSA Rouen, UNIROUEN, F-76000 Rouen, France |
推荐引用方式 GB/T 7714 | Wu, Junteng,Faccinetto, Alessandro,Grimonprez, Symphorien,et al. Influence of the dry aerosol particle size distribution and morphology on the cloud condensation nuclei activation. An experimental and theoretical investigation[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2020,20(7):4209-4225. |
APA | Wu, Junteng.,Faccinetto, Alessandro.,Grimonprez, Symphorien.,Batut, Sebastien.,Yon, Jerome.,...&Petitprez, Denis.(2020).Influence of the dry aerosol particle size distribution and morphology on the cloud condensation nuclei activation. An experimental and theoretical investigation.ATMOSPHERIC CHEMISTRY AND PHYSICS,20(7),4209-4225. |
MLA | Wu, Junteng,et al."Influence of the dry aerosol particle size distribution and morphology on the cloud condensation nuclei activation. An experimental and theoretical investigation".ATMOSPHERIC CHEMISTRY AND PHYSICS 20.7(2020):4209-4225. |
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