资源环境科技发展态势分析平台

We investigated the climatological-scale, monthly binned, seasonal variation of AERONET/Dubovik retrievals across six stations in the North American and European Arctic (multiyear sampling periods ranging from 8 to 17 years). A robust, spring-to-summer (StoS) increase in the radius of the peak of the fine mode (FM) component of the particle size distribution (PSD) was observed for five of the six stations. The FM aerosol optical depth (AOD) and the FM effective radius at the individual stations showed, respectively, a negligible to moderate StoS decrease and a significant increase. This was interpreted as a trade-off between the waning influence of smaller FM Arctic haze aerosols and the increasing influence of large FM smoke particles. A springtime, pan-Arctic PSD peak in the 1.3 mu m coarse mode (CM) bin was attributed to Asian dust. It was suggested that the increase in amplitude of a second (4-7 mu m) CM peak from July to August at the low-elevation coastal sites was influenced by wind-induced sea salt. The CM AOD went through a StoS decrease attributed to the decreasing amplitude of the 1.3 mu m peak. A significant StoS CM effective radius increase was ascribed to the decreasing influence of the 1.3 mu m peak. StoS FM fraction increases were largely due to the decrease of the CM AOD (decreasing influence of springtime Asian dust). This extensive and intensive climatology of remotely sensed, bimodal properties will, we believe, provide an important reference for future measurements and modeling of Arctic aerosols.