Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.5194/acp-13-7405-2013 |
ACE-FTS observations of acetonitrile in the lower stratosphere | |
J. J. Harrison and P. F. Bernath | |
2013-08-02 | |
发表期刊 | Atmospheric Chemistry and Physics
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出版年 | 2013 |
英文摘要 | This work reports the first infrared satellite remote-sensing measurements of acetonitrile (CH3CN) in the Earth's atmosphere using solar occultation measurements made by the Atmospheric Chemistry Experiment Fourier transform spectrometer (ACE-FTS) between 2004 and 2011. The retrieval scheme uses new quantitative laboratory spectroscopic measurements of acetonitrile (Harrison and Bernath, 2012). Although individual ACE-FTS profile measurements are dominated by measurement noise, median profiles in 10° latitude bins show a steady decline in volume mixing ratio from ~150 ppt (parts per trillion) at 11.5 km to < 40 ppt at 25.5–29.5 km. These new measurements agree well with the scant available air- and balloon-borne data in the lower stratosphere. An acetonitrile stratospheric lifetime of 73 ± 20 yr has been determined. |
领域 | 地球科学 |
URL | 查看原文 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/288034 |
专题 | 地球科学 |
推荐引用方式 GB/T 7714 | J. J. Harrison and P. F. Bernath. ACE-FTS observations of acetonitrile in the lower stratosphere[J]. Atmospheric Chemistry and Physics,2013. |
APA | J. J. Harrison and P. F. Bernath.(2013).ACE-FTS observations of acetonitrile in the lower stratosphere.Atmospheric Chemistry and Physics. |
MLA | J. J. Harrison and P. F. Bernath."ACE-FTS observations of acetonitrile in the lower stratosphere".Atmospheric Chemistry and Physics (2013). |
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