Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.5194/acp-17-1297-2017 |
Influence of enhanced Asian NOx emissions on ozone in the upper troposphere and lower stratosphere in chemistry-climate model simulations | |
Roy, Chaitri1; Fadnavis, Suvarna1; Mueller, Rolf2; Ayantika, D. C.1; Ploeger, Felix2; Rap, Alexandru3 | |
2017-01-27 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS
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ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2017 |
卷号 | 17期号:2 |
文章类型 | Article |
语种 | 英语 |
国家 | India; Germany; England |
英文摘要 | The Asian summer monsoon (ASM) anticyclone is the most pronounced circulation pattern in the upper troposphere and lower stratosphere (UTLS) during northern hemispheric summer. ASM convection plays an important role in efficient vertical transport from the surface to the upper-level anticyclone. In this paper we investigate the potential impact of enhanced anthropogenic nitrogen oxide (NOx) emissions on the distribution of ozone in the UTLS using the fully coupled aerosol-chemistry-climate model, ECHAM5-HAMMOZ. Ozone in the UTLS is influenced both by the convective uplift of ozone precursors and by the uplift of enhanced-NOx-induced tropospheric ozone anomalies. We performed anthropogenic NOx emission sensitivity experiments over India and China. In these simulations, covering the years 2000-2010, anthropogenic NOx emissions have been increased by 38% over India and by 73% over China with respect to the emission base year 2000. These emission increases are comparable to the observed linear trends of 3.8% per year over India and 7.3% per year over China during the period 2000 to 2010. Enhanced NOx emissions over India by 38% and China by 73% increase the ozone radiative forcing in the ASM anticyclone (15-40 degrees N, 60-120 degrees E) by 16.3 and 78.5mW m(-2) respectively. These elevated NOx emissions produce significant warming over the Tibetan Plateau and increase precipitation over India due to a strengthening of the monsoon Hadley circulation. However, increase in NOx emissions over India by 73% (similar to the observed increase over China) results in large ozone production over the Indo-Gangetic Plain and Tibetan Plateau. The higher ozone concentrations, in turn, induce a reversed monsoon Hadley circulation and negative precipitation anomalies over India. The associated subsidence suppresses vertical transport of NOx and ozone into the ASM anticyclone. |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000394604000004 |
WOS关键词 | INDIAN-SUMMER MONSOON ; SEASONAL-VARIATION ; WATER-VAPOR ; NITROGEN-OXIDES ; SURFACE OZONE ; INTERANNUAL VARIABILITY ; SATELLITE-OBSERVATIONS ; ATMOSPHERIC CHEMISTRY ; PEROXYACETYL NITRATE ; TRANSPORT PATHWAYS |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/30388 |
专题 | 地球科学 |
作者单位 | 1.Indian Inst Trop Meteorol, Pune, Maharashtra, India; 2.Forschungszentrum Julich, IEK7, Julich, Germany; 3.Univ Leeds, Sch Earth & Environm, Leeds, W Yorkshire, England |
推荐引用方式 GB/T 7714 | Roy, Chaitri,Fadnavis, Suvarna,Mueller, Rolf,et al. Influence of enhanced Asian NOx emissions on ozone in the upper troposphere and lower stratosphere in chemistry-climate model simulations[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2017,17(2). |
APA | Roy, Chaitri,Fadnavis, Suvarna,Mueller, Rolf,Ayantika, D. C.,Ploeger, Felix,&Rap, Alexandru.(2017).Influence of enhanced Asian NOx emissions on ozone in the upper troposphere and lower stratosphere in chemistry-climate model simulations.ATMOSPHERIC CHEMISTRY AND PHYSICS,17(2). |
MLA | Roy, Chaitri,et al."Influence of enhanced Asian NOx emissions on ozone in the upper troposphere and lower stratosphere in chemistry-climate model simulations".ATMOSPHERIC CHEMISTRY AND PHYSICS 17.2(2017). |
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