Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.5194/acp-19-3065-2019 |
Transport of Po Valley aerosol pollution to the northwestern Alps Part 1: Phenomenology | |
Diemoz, Henri1; Barnaba, Francesca2; Magri, Tiziana1; Pession, Giordano1; Dionisi, Davide2; Pittavino, Sara1; Tombolato, Ivan K. F.1; Campanelli, Monica2; Sofia Della Ceca, Lara3; Hervo, Maxime4; Di Liberto, Luca2; Ferrero, Luca5,6; Gobbi, Gian Paolo2 | |
2019-03-11 | |
发表期刊 | ATMOSPHERIC CHEMISTRY AND PHYSICS
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ISSN | 1680-7316 |
EISSN | 1680-7324 |
出版年 | 2019 |
卷号 | 19期号:5页码:3065-3095 |
文章类型 | Article |
语种 | 英语 |
国家 | Italy; Argentina; Switzerland |
英文摘要 | Mountainous regions are often considered pristine environments; however they can be affected by pollutants emitted in more populated and industrialised areas, transported by regional winds. Based on experimental evidence, further supported by modelling tools, here we demonstrate and quantify the impact of air masses transported from the Po Valley, a European atmospheric pollution hotspot, to the northwestern Alps. This is achieved through a detailed investigation of the phenomenology of near-range (a few hundred kilometres), trans-regional transport, exploiting synergies of multi-sensor observations mainly focussed on particulate matter. The explored dataset includes vertically resolved data from atmospheric profiling techniques (automated lidar ceilometers, ALCs), vertically integrated aerosol properties from ground (sun photometer) and space, and in situ measurements (PM10 and PM2.5, relevant chemical analyses, and aerosol size distribution). During the frequent advection episodes from the Po basin, all the physical quantities observed by the instrumental setup are found to significantly increase: the scattering ratio from ALC reaches values > 30, aerosol optical depth (AOD) triples, surface PM10 reaches concentrations > 100 mu gm(-3) even in rural areas, and contributions to PM10 by secondary inorganic compounds such as nitrate, ammonium, and sulfate increase up to 28 %, 8 %, and 17 %, respectively. Results also indicate that the aerosol advected from the Po Valley is hygroscopic, smaller in size, and less light-absorbing compared to the aerosol type locally emitted in the northwestern Italian Alps. In this work, the phenomenon is exemplified through detailed analysis and discussion of three case studies, selected for their clarity and relevance within the wider dataset, the latter being fully exploited in a companion paper quantifying the impact of this phenomenology over the long-term (Diemoz et al., 2019). For the three case studies investigated, a high-resolution numerical weather prediction model (COSMO) and a Lagrangian tool (LAGRANTO) are employed to understand the meteorological mechanisms favouring transport and to demonstrate the Po Valley origin of the air masses. In addition, a chemical transport model (FARM) is used to further support the observations and to partition the contributions of local and non-local sources. Results show that the simulations are important to the understanding of the phenomenon under investigation. However, in quantitative terms, modelled PM10 concentrations are 4-5 times lower than the ones retrieved from the ALC and maxima are anticipated in time by 6-7 h. Underestimated concentrations are likely mainly due to deficiencies in the emission inventory and to water uptake of the advected particles not fully reproduced by FARM, while timing mismatches are likely an effect of suboptimal simulation of up-valley and down-valley winds by COSMO. The advected aerosol is shown to remarkably degrade the air quality of the Alpine region, with potential negative effects on human health, climate, and ecosystems, as well as on the touristic development of the investigated area. The findings of the present study could also help design mitigation strategies at the trans-regional scale in the Po basin and suggest an observation-based approach to evaluate the outcome of their implementation. |
领域 | 地球科学 |
收录类别 | SCI-E |
WOS记录号 | WOS:000460839900002 |
WOS关键词 | SECONDARY ORGANIC AEROSOL ; REGIONAL BACKGROUND SITE ; HEAT-TRANSFER PROCESSES ; AIR-POLLUTION ; PARTICULATE MATTER ; CHEMICAL-COMPOSITION ; OPTICAL-PROPERTIES ; IN-SITU ; LIDAR OBSERVATIONS ; SIZE DISTRIBUTION |
WOS类目 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/30661 |
专题 | 地球科学 |
作者单位 | 1.ARPA Valle Aosta, St Christophe, Italy; 2.ISAC CNR, Inst Atmospher Sci & Climate, Rome, Italy; 3.Inst Fis Rosario, Rosario, Santa Fe, Argentina; 4.MeteoSwiss, Payerne, Switzerland; 5.Univ Milano Bicocca, GEMMA Res Ctr, Milan, Italy; 6.Univ Milano Bicocca, POLARIS Res Ctr, Dept Earth & Environm Sci, Milan, Italy |
推荐引用方式 GB/T 7714 | Diemoz, Henri,Barnaba, Francesca,Magri, Tiziana,et al. Transport of Po Valley aerosol pollution to the northwestern Alps Part 1: Phenomenology[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019,19(5):3065-3095. |
APA | Diemoz, Henri.,Barnaba, Francesca.,Magri, Tiziana.,Pession, Giordano.,Dionisi, Davide.,...&Gobbi, Gian Paolo.(2019).Transport of Po Valley aerosol pollution to the northwestern Alps Part 1: Phenomenology.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(5),3065-3095. |
MLA | Diemoz, Henri,et al."Transport of Po Valley aerosol pollution to the northwestern Alps Part 1: Phenomenology".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.5(2019):3065-3095. |
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