GSTDTAP  > 地球科学
DOI10.5194/acp-19-3557-2019
Saharan dust and biomass burning aerosols during ex-hurricane Ophelia: observations from the new UK lidar and sun-photometer network
Osborne, Martin1,2; Malavelle, Florent F.2; Adam, Mariana3; Buxmann, Joelle1; Sugier, Jaqueline1; Marenco, Franco1; Haywood, Jim1,2
2019-03-20
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2019
卷号19期号:6页码:3557-3578
文章类型Article
语种英语
国家England; Romania
英文摘要

On 15-16 October 2017, ex-hurricane Ophelia passed to the west of the British Isles, bringing dust from the Sahara and smoke from Portuguese forest fires that was observable to the naked eye and reported in the UK's national press. We report here detailed observations of this event using the UK operational lidar and sun-photometer network, established for the early detection of aviation hazards, including volcanic ash. We also use ECMWF ERA5 wind field data and MODIS imagery to examine the aerosol transport. The observations, taken continuously over a period of 30 h, show a complex picture, dominated by several different aerosol layers at different times and clearly correlated with the passage of different air masses associated with the intense cyclonic system. A similar evolution was observed at several sites, with a time delay between them explained by their different location with respect to the storm and associated meteorological features. The event commenced with a shallow dust layer at 1-2 km in altitude and culminated in a deep and complex structure that lasted similar to 12 h at each site over the UK, correlated with the storm's warm sector. For most of the time, the aerosol detected was dominated by mineral dust mixtures, as highlighted by depolarisation measurements, but an intense biomass burning aerosol (BBA) layer was observed towards the end of the event, lasting around 3 h at each site. The aerosol optical depth at 355 nm (AOD(355)) during the whole event ranged from 0.2 to 2.9, with the larger AOD correlated to the intense BBA layer. Such a large AOD is unprecedented in the UK according to AERONET records for the last 20 years. The Raman lidars permitted the measurement of the aerosol extinction coefficient at 355 nm, the particle linear depolarisation ratio (PLDR), and the lidar ratio (LR) and made the separation of the dust (depolarising) aerosol from other aerosol types possible. A specific extinction has also been computed to provide an estimate of the atmospheric concentration of both aerosol types separately, which peaked at 420 +/- 200 mu g m(-3) for the dust and 558 +/- 232 mu g m(-3) for the biomass burning aerosols. Back trajectories computed using the Numerical Atmospheric-dispersion Modelling Environment (NAME) were used to identify the sources and strengthen the conclusions drawn from the observations. The UK network represents a significant expansion of the observing capability in northern Europe, with instruments evenly distributed across Great Britain, from Camborne in Cornwall to Lerwick in the Shetland Islands, and this study represents the first attempt to demonstrate its capability and validate the methods in use. Its ultimate purpose will be the detection and quantification of volcanic plumes, but the present study clearly demonstrates the advanced capabilities of the network.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000461894100002
WOS关键词COMPLEX REFRACTIVE-INDEX ; SINGLE CALCULUS CHAIN ; IN-SITU MEASUREMENTS ; OPTICAL-PROPERTIES ; DEPOLARIZATION RATIO ; MINERAL DUST ; MICROPHYSICAL PROPERTIES ; EXTINCTION PROFILES ; UNITED-KINGDOM ; VOLCANIC ASH
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/31068
专题地球科学
作者单位1.Met Off, Fitzroy Rd, Exeter EX1 3PB, Devon, England;
2.Univ Exeter, Laver Bldg,North Pk Rd, Exeter EX4 4QE, Devon, England;
3.Natl Inst R&D Optoelect INOE2000, Str Atomistilor 409, Magurele 077125, Ilfov, Romania
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GB/T 7714
Osborne, Martin,Malavelle, Florent F.,Adam, Mariana,et al. Saharan dust and biomass burning aerosols during ex-hurricane Ophelia: observations from the new UK lidar and sun-photometer network[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2019,19(6):3557-3578.
APA Osborne, Martin.,Malavelle, Florent F..,Adam, Mariana.,Buxmann, Joelle.,Sugier, Jaqueline.,...&Haywood, Jim.(2019).Saharan dust and biomass burning aerosols during ex-hurricane Ophelia: observations from the new UK lidar and sun-photometer network.ATMOSPHERIC CHEMISTRY AND PHYSICS,19(6),3557-3578.
MLA Osborne, Martin,et al."Saharan dust and biomass burning aerosols during ex-hurricane Ophelia: observations from the new UK lidar and sun-photometer network".ATMOSPHERIC CHEMISTRY AND PHYSICS 19.6(2019):3557-3578.
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