GSTDTAP  > 气候变化
DOI10.1029/2018JD028768
Modeling of Atmospheric Aerosol Properties in the SAo Paulo Metropolitan Area: Impact of Biomass Burning
Vara-Vela, Angel1; Andrade, Maria de Fatima1; Zhang, Yang2; Kumar, Prashant3,4; Ynoue, Rita Yuri1; Souto-Oliveira, Carlos Eduardo5; da Silva Lopes, Fabio Juliano1,6; Landulfo, Eduardo6
2018-09-16
发表期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
EISSN2169-8996
出版年2018
卷号123期号:17页码:9935-9956
文章类型Article
语种英语
国家Brazil; USA; England
英文摘要

Smoke particles ejected into the atmosphere from biomass burning can modify the atmospheric composition around and even far from the sources. In late winter and early spring, biomass burning emissions from inland regions can be efficiently transported to urban areas in southeastern South America, thus affecting air quality in those areas. In this study, the Weather Research and Forecasting with Chemistry model was applied in order to investigate the impact of biomass burning sources on aerosol loadings and properties over the SAo Paulo Metropolitan Area (SPMA), in southeastern Brazil, during the period from 19 August to 3 September 2014. The model performance was evaluated using available aerosol measurements from the Narrowing the Uncertainties on Aerosol and Climate Change in SAo Paulo State project. The combined application of aerosol data and Weather Research and Forecasting with Chemistry simulations made it possible to represent some of the most important aerosol properties, such as particle number concentration and cloud condensation nuclei activation, in addition to evaluation of the impact of biomass burning by analyzing a 5-day transport event, from 22 to 26 August 2014. During this transport event, differences in the average predicted PM2.5 concentration reached 15g/m(3) (peaking at 20g/m(3) during the nighttime hours) over the SPMA, compared with 35g/m(3) over inland areas northwest and north of the SPMA. Biomass burning accounted for up to 20% of the baseline particle number concentration- and cloud condensation nuclei-weighted relative differences over the SPMA (2,300 and 1,400cm(-3), respectively).


领域气候变化
收录类别SCI-E
WOS记录号WOS:000445617500058
WOS关键词SECONDARY ORGANIC AEROSOL ; CLOUD CONDENSATION NUCLEI ; REGIONAL AIR-QUALITY ; WRF-CHEM MODEL ; SOURCE APPORTIONMENT ; PARTICULATE MATTER ; PARTICLE FORMATION ; WEATHER FORECASTS ; ABSORPTION-MODEL ; AMAZON REGION
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/32837
专题气候变化
作者单位1.Univ Sao Paulo, Inst Astron Geophys & Atmospher Sci, Dept Atmospher Sci, Sao Paulo, Brazil;
2.North Carolina State Univ, Dept Marine Earth & Atmospher Sci, Coll Sci, Raleigh, NC USA;
3.Univ Surrey, Fac Engn & Phys Sci, Dept Civil & Environm Engn, Global Ctr Clean Air Res, Guildford, Surrey, England;
4.Univ Surrey, Fac Engn & Phys Sci, Environm Flow Res Ctr, Guildford, Surrey, England;
5.Univ Sao Paulo, Inst Geosci, Geocronol Res Ctr, Sao Paulo, Brazil;
6.Nucl & Energy Res Inst, Ctr Laser & Applicat, Sao Paulo, Brazil
推荐引用方式
GB/T 7714
Vara-Vela, Angel,Andrade, Maria de Fatima,Zhang, Yang,et al. Modeling of Atmospheric Aerosol Properties in the SAo Paulo Metropolitan Area: Impact of Biomass Burning[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2018,123(17):9935-9956.
APA Vara-Vela, Angel.,Andrade, Maria de Fatima.,Zhang, Yang.,Kumar, Prashant.,Ynoue, Rita Yuri.,...&Landulfo, Eduardo.(2018).Modeling of Atmospheric Aerosol Properties in the SAo Paulo Metropolitan Area: Impact of Biomass Burning.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,123(17),9935-9956.
MLA Vara-Vela, Angel,et al."Modeling of Atmospheric Aerosol Properties in the SAo Paulo Metropolitan Area: Impact of Biomass Burning".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 123.17(2018):9935-9956.
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