Global S&T Development Trend Analysis Platform of Resources and Environment
DOI | 10.1029/2018JD028647 |
Vertical Profiles of Tropospheric Ozone From MAX-DOAS Measurements During the CINDI-2 Campaign: Part 1Development of a New Retrieval Algorithm | |
Wang, Yang1; Pukite, Janis1; Wagner, Thomas1; Donner, Sebastian1; Beirle, Steffen1; Hilboll, Andreas2; Vrekoussis, Mihalis2,3; Richter, Andreas2; Apituley, Arnoud4; Piters, Ankie4; Allaart, Marc4; Eskes, Henk4; Frumau, Arnoud5; Van Roozendael, Michel6; Lampel, Johannes7; Platt, Ulrich7; Schmitt, Stefan7; Swart, Daan8; Vonk, Jan8 | |
2018-09-27 | |
发表期刊 | JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
![]() |
ISSN | 2169-897X |
EISSN | 2169-8996 |
出版年 | 2018 |
卷号 | 123期号:18页码:10637-10670 |
文章类型 | Article |
语种 | 英语 |
国家 | Germany; Cyprus; Netherlands; Belgium |
英文摘要 | Ground-based measurements of tropospheric ozone (O-3) are valuable for studies of atmospheric chemistry, air pollution, climate change, and for satellite validation. The Multi Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) technique has been widely used to derive vertical profiles of trace gases and aerosols in the troposphere. However, tropospheric O-3 has not yet been satisfactorily derived from MAX-DOAS measurements due to the influence of stratospheric O-3 absorption. In this study, we developed two new retrieval approaches for tropospheric O-3 from MAX-DOAS measurements. In method 1, stratospheric O-3 profiles from external data sources are considered in the retrieval. In method 2, stratospheric and tropospheric O-3 are separated based on the temperature-dependent differences between tropospheric and stratospheric O-3 absorption structures in the UV spectral range. The feasibility of both methods is first verified by applying them to synthetic spectra. Then they are applied to real MAX-DOAS measurements recorded during the CINDI-2 campaign in Cabauw, the Netherlands (September 2016). The obtained results are compared with independent O-3 measurements and global chemical transport model simulations. Good agreement of the near-surface O-3 concentrations with the independent data sets is found for both methods. However, tropospheric O-3 profiles are only reasonably derived using method 1, while they are significantly overestimated at altitudes above 1km using method 2, probably due to the approximation of the ring spectra used to correct the rotational Raman scattering structures in the DOAS fit. Advantages and disadvantages of both methods are discussed and improvement directions are suggested for further studies. |
英文关键词 | tropospheric ozone vertical profile MAX-DOAS |
领域 | 气候变化 |
收录类别 | SCI-E |
WOS记录号 | WOS:000447807300035 |
WOS关键词 | OPTICAL-ABSORPTION SPECTROSCOPY ; RADIATIVE-TRANSFER MODEL ; AEROSOL EXTINCTION ; ATMOSPHERIC AEROSOLS ; DERIVE INFORMATION ; RAMAN-SCATTERING ; CROSS-SECTIONS ; O-4 ABSORPTION ; NO2 ; AIR |
WOS类目 | Meteorology & Atmospheric Sciences |
WOS研究方向 | Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/33291 |
专题 | 气候变化 |
作者单位 | 1.Max Planck Inst Chem, Mainz, Germany; 2.Univ Bremen, Inst Environm Phys, Bremen, Germany; 3.Cyprus Inst, Nicosia, Cyprus; 4.Royal Netherlands Meteorol Inst, De Bilt, Netherlands; 5.Energy Res Ctr Netherlands, Petten, Netherlands; 6.Royal Belgian Inst Space Aeron BIRA IASB, Brussels, Belgium; 7.Heidelberg Univ, Inst Environm Phys, Heidelberg, Germany; 8.Natl Inst Publ Hlth & Environm, Bilthaven, Netherlands |
推荐引用方式 GB/T 7714 | Wang, Yang,Pukite, Janis,Wagner, Thomas,et al. Vertical Profiles of Tropospheric Ozone From MAX-DOAS Measurements During the CINDI-2 Campaign: Part 1Development of a New Retrieval Algorithm[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2018,123(18):10637-10670. |
APA | Wang, Yang.,Pukite, Janis.,Wagner, Thomas.,Donner, Sebastian.,Beirle, Steffen.,...&Vonk, Jan.(2018).Vertical Profiles of Tropospheric Ozone From MAX-DOAS Measurements During the CINDI-2 Campaign: Part 1Development of a New Retrieval Algorithm.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,123(18),10637-10670. |
MLA | Wang, Yang,et al."Vertical Profiles of Tropospheric Ozone From MAX-DOAS Measurements During the CINDI-2 Campaign: Part 1Development of a New Retrieval Algorithm".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 123.18(2018):10637-10670. |
条目包含的文件 | 条目无相关文件。 |
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。
修改评论