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DOI10.1002/2017JD027833
Numerical Investigation on Absorption Enhancement of Black Carbon Aerosols Partially Coated With Nonabsorbing Organics
Zhang, Xiaolin1,2,3; Mao, Mao1,2,3; Yin, Yan1,2; Wang, Bin1,3
2018-01-27
发表期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
EISSN2169-8996
出版年2018
卷号123期号:2页码:1297-1308
文章类型Article
语种英语
国家Peoples R China; USA
英文摘要

This study numerically evaluates the effects of aerosol microphysics, including coated volume fraction of black carbon (BC), shell/core ratio, and size distribution, on the absorption enhancement (E-ab) of polydisperse BC aggregates partially coated by organics, which is calculated by the exact multiple-sphere T-matrix method. The coated volume fraction of BC plays a substantial role in determining the absorption enhancement of partially coated BC aggregates, which typically have an E-ab in the range of similar to 1.0-2.0 with a larger value for larger coated volume fraction of BC as the shell/core ratio, BC geometry, and size distribution are fixed. The shell/core ratio, BC geometry, and size distribution have little impact on the E-ab of coated BC with small coated volume fraction of BC, while they become significant for large coated volume fraction of BC. The E-ab of partially coated BC particles can be slightly less than 1.0 for the large BC in the accumulation mode exhibiting large shell/core ratio and small coated volume fraction of BC, indicating that the absorption shows even slight decrease relative to uncoated BC particles. For partially coated BC aggregates in the accumulation and coarse modes, the refractive index uncertainties of BC result in the E-ab differences of less than 9% and 2%, respectively, while those of organics can induce larger variations with the maximum differences up to 22% and 18%, respectively. Our study indicates that accounting for particle coating microphysics, particularly the coated volume fraction of BC, can potentially help to understand the differences in observations of largely variable absorption enhancements over various regions.


英文关键词black carbon aerosol absorption enhancement partial coating numerical investigation
领域气候变化
收录类别SCI-E
WOS记录号WOS:000425520200039
WOS关键词DISCRETE-DIPOLE APPROXIMATION ; LIGHT-ABSORPTION ; OPTICAL-PROPERTIES ; RADIATIVE PROPERTIES ; SOOT AEROSOLS ; BROWN CARBON ; T-MATRIX ; CROSS-SECTION ; MIXING STATES ; URBAN HAZE
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/33607
专题气候变化
作者单位1.Nanjing Univ Informat Sci & Technol, Earth Syst Modeling Ctr,Collaborat Innovat Ctr Fo, Key Lab Aerosol Cloud Precipitat,China Meteorol A, Joint Int Res Lab Climate & Environm Change,Key L, Nanjing, Jiangsu, Peoples R China;
2.Nanjing Univ Informat Sci & Technol, Sch Atmospher Phys, Nanjing, Jiangsu, Peoples R China;
3.Univ Hawaii Manoa, Int Pacific Res Ctr, Honolulu, HI 96822 USA
推荐引用方式
GB/T 7714
Zhang, Xiaolin,Mao, Mao,Yin, Yan,et al. Numerical Investigation on Absorption Enhancement of Black Carbon Aerosols Partially Coated With Nonabsorbing Organics[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2018,123(2):1297-1308.
APA Zhang, Xiaolin,Mao, Mao,Yin, Yan,&Wang, Bin.(2018).Numerical Investigation on Absorption Enhancement of Black Carbon Aerosols Partially Coated With Nonabsorbing Organics.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,123(2),1297-1308.
MLA Zhang, Xiaolin,et al."Numerical Investigation on Absorption Enhancement of Black Carbon Aerosols Partially Coated With Nonabsorbing Organics".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 123.2(2018):1297-1308.
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