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DOI | 10.1002/2017JD027833 |
Numerical Investigation on Absorption Enhancement of Black Carbon Aerosols Partially Coated With Nonabsorbing Organics | |
Zhang, Xiaolin1,2,3; Mao, Mao1,2,3; Yin, Yan1,2; Wang, Bin1,3 | |
2018-01-27 | |
发表期刊 | JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
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ISSN | 2169-897X |
EISSN | 2169-8996 |
出版年 | 2018 |
卷号 | 123期号:2页码:1297-1308 |
文章类型 | Article |
语种 | 英语 |
国家 | Peoples R China; USA |
英文摘要 | This study numerically evaluates the effects of aerosol microphysics, including coated volume fraction of black carbon (BC), shell/core ratio, and size distribution, on the absorption enhancement (E-ab) of polydisperse BC aggregates partially coated by organics, which is calculated by the exact multiple-sphere T-matrix method. The coated volume fraction of BC plays a substantial role in determining the absorption enhancement of partially coated BC aggregates, which typically have an E-ab in the range of similar to 1.0-2.0 with a larger value for larger coated volume fraction of BC as the shell/core ratio, BC geometry, and size distribution are fixed. The shell/core ratio, BC geometry, and size distribution have little impact on the E-ab of coated BC with small coated volume fraction of BC, while they become significant for large coated volume fraction of BC. The E-ab of partially coated BC particles can be slightly less than 1.0 for the large BC in the accumulation mode exhibiting large shell/core ratio and small coated volume fraction of BC, indicating that the absorption shows even slight decrease relative to uncoated BC particles. For partially coated BC aggregates in the accumulation and coarse modes, the refractive index uncertainties of BC result in the E-ab differences of less than 9% and 2%, respectively, while those of organics can induce larger variations with the maximum differences up to 22% and 18%, respectively. Our study indicates that accounting for particle coating microphysics, particularly the coated volume fraction of BC, can potentially help to understand the differences in observations of largely variable absorption enhancements over various regions. |
英文关键词 | black carbon aerosol absorption enhancement partial coating numerical investigation |
领域 | 气候变化 |
收录类别 | SCI-E |
WOS记录号 | WOS:000425520200039 |
WOS关键词 | DISCRETE-DIPOLE APPROXIMATION ; LIGHT-ABSORPTION ; OPTICAL-PROPERTIES ; RADIATIVE PROPERTIES ; SOOT AEROSOLS ; BROWN CARBON ; T-MATRIX ; CROSS-SECTION ; MIXING STATES ; URBAN HAZE |
WOS类目 | Meteorology & Atmospheric Sciences |
WOS研究方向 | Meteorology & Atmospheric Sciences |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://119.78.100.173/C666/handle/2XK7JSWQ/33607 |
专题 | 气候变化 |
作者单位 | 1.Nanjing Univ Informat Sci & Technol, Earth Syst Modeling Ctr,Collaborat Innovat Ctr Fo, Key Lab Aerosol Cloud Precipitat,China Meteorol A, Joint Int Res Lab Climate & Environm Change,Key L, Nanjing, Jiangsu, Peoples R China; 2.Nanjing Univ Informat Sci & Technol, Sch Atmospher Phys, Nanjing, Jiangsu, Peoples R China; 3.Univ Hawaii Manoa, Int Pacific Res Ctr, Honolulu, HI 96822 USA |
推荐引用方式 GB/T 7714 | Zhang, Xiaolin,Mao, Mao,Yin, Yan,et al. Numerical Investigation on Absorption Enhancement of Black Carbon Aerosols Partially Coated With Nonabsorbing Organics[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2018,123(2):1297-1308. |
APA | Zhang, Xiaolin,Mao, Mao,Yin, Yan,&Wang, Bin.(2018).Numerical Investigation on Absorption Enhancement of Black Carbon Aerosols Partially Coated With Nonabsorbing Organics.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,123(2),1297-1308. |
MLA | Zhang, Xiaolin,et al."Numerical Investigation on Absorption Enhancement of Black Carbon Aerosols Partially Coated With Nonabsorbing Organics".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 123.2(2018):1297-1308. |
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