GSTDTAP
项目编号1506691
Laboratory Studies of Contact Efflorescence
Margaret Tolbert
主持机构University of Colorado at Boulder
项目开始年2015
2015-08-15
项目结束日期2018-07-31
资助机构US-NSF
项目类别Standard Grant
项目经费438404(USD)
国家美国
语种英语
英文摘要As atmospheric relative humidity cycles, saline aerosols exist either as ionic salts, or as aqueous ionic solution. Supersaturated and undersaturated phase change typically demonstrate hysteresis behavior as a function of relative humidity. The (increasing) RH at which the phase transition abruptly changes from solid particle to a saturated aqueous solution is the deliquescence relative humidity (DRH). The decreasing RH that drying aqueous droplets remain as supersaturated sols until crystallization, is the efflorescence relative humidity (ERH). Efflorescence may differ based on the nucleation mechanism, either by contact with a seed, or immersion of that seed into the supersaturated droplet. The objective of a series of laboratory investigations is to further study contact efflorescence compared to immersion efflorescence on aerosol types and sizes representative of atmospheric particles. Aerosol phase changes in a single droplet optical trap will be used to systematically follow efflorescence mechanisms.

The importance of accounting for aerosol particle phase changes includes effects on heterogeneous chemical processes, light scattering, and cloud formation and precipitation. Direct effects on homogeneous (gas phase) chemistry and climate also remain uncertain.
来源学科分类Geosciences - Atmospheric and Geospace Sciences
文献类型项目
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/68500
专题环境与发展全球科技态势
推荐引用方式
GB/T 7714
Margaret Tolbert.Laboratory Studies of Contact Efflorescence.2015.
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