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CO2 Dissolution Trapping Rates in Heterogeneous Porous Media 期刊论文
GEOPHYSICAL RESEARCH LETTERS, 2020, 47 (12)
作者:  Gilmore, K. A.;  Neufeld, J. A.;  Bickle, M. J.
收藏  |  浏览/下载:23/0  |  提交时间:2020/06/01
geological carbon storage  dissolution trapping  heterogeneous porous media  
Observation of Bose-Einstein condensates in an Earth-orbiting research lab 期刊论文
NATURE, 2020, 582 (7811) : 103-+
作者:  Yamamoto, Keisuke;  Venida, Anthony;  Yano, Julian;  Biancur, Douglas E.;  Kakiuchi, Miwako;  Gupta, Suprit;  Sohn, Albert S. W.;  Mukhopadhyay, Subhadip;  Lin, Elaine Y.;  Parker, Seth J.;  Banh, Robert S.;  Paulo, Joao A.;  Wen, Kwun Wah;  Debnath, Jayanta;  Kim, Grace E.;  Mancias, Joseph D.;  Fearon, Douglas T.;  Perera, Rushika M.;  Kimmelman, Alec C.
收藏  |  浏览/下载:46/0  |  提交时间:2020/07/03

Quantum mechanics governs the microscopic world, where low mass and momentum reveal a natural wave-particle duality. Magnifying quantum behaviour to macroscopic scales is a major strength of the technique of cooling and trapping atomic gases, in which low momentum is engineered through extremely low temperatures. Advances in this field have achieved such precise control over atomic systems that gravity, often negligible when considering individual atoms, has emerged as a substantial obstacle. In particular, although weaker trapping fields would allow access to lower temperatures(1,2), gravity empties atom traps that are too weak. Additionally, inertial sensors based on cold atoms could reach better sensitivities if the free-fall time of the atoms after release from the trap could be made longer(3). Planetary orbit, specifically the condition of perpetual free-fall, offers to lift cold-atom studies beyond such terrestrial limitations. Here we report production of rubidium Bose-Einstein condensates (BECs) in an Earth-orbiting research laboratory, the Cold Atom Lab. We observe subnanokelvin BECs in weak trapping potentials with free-expansion times extending beyond one second, providing an initial demonstration of the advantages offered by a microgravity environment for cold-atom experiments and verifying the successful operation of this facility. With routine BEC production, continuing operations will support long-term investigations of trap topologies unique to microgravity(4,5), atom-laser sources(6), few-body physics(7,8)and pathfinding techniques for atom-wave interferometry(9-12).


  
Performance-limiting nanoscale trap clusters at grain junctions in halide perovskites 期刊论文
NATURE, 2020, 580 (7803) : 360-+
作者:  van den Brink, Susanne C.;  Alemany, Anna;  van Batenburg, Vincent;  Moris, Naomi;  Blotenburg, Marloes;  Vivie, Judith;  Baillie-Johnson, Peter;  Nichols, Jennifer;  Sonnen, Katharina F.;  Arias, Alfonso;  van Oudenaarden, Alexander
收藏  |  浏览/下载:38/0  |  提交时间:2020/07/03

Halide perovskite materials have promising performance characteristics for low-cost optoelectronic applications. Photovoltaic devices fabricated from perovskite absorbers have reached power conversion efficiencies above 25 per cent in single-junction devices and 28 per cent in tandem devices(1,2). This strong performance (albeit below the practical limits of about 30 per cent and 35 per cent, respectively(3)) is surprising in thin films processed from solution at low-temperature, a method that generally produces abundant crystalline defects(4). Although point defects often induce only shallow electronic states in the perovskite bandgap that do not affect performance(5), perovskite devices still have many states deep within the bandgap that trap charge carriers and cause them to recombine non-radiatively. These deep trap states thus induce local variations in photoluminescence and limit the device performance(6). The origin and distribution of these trap states are unknown, but they have been associated with light-induced halide segregation in mixed-halide perovskite compositions(7) and with local strain(8), both of which make devices less stable(9). Here we use photoemission electron microscopy to image the trap distribution in state-of-the-art halide perovskite films. Instead of a relatively uniform distribution within regions of poor photoluminescence efficiency, we observe discrete, nanoscale trap clusters. By correlating microscopy measurements with scanning electron analytical techniques, we find that these trap clusters appear at the interfaces between crystallographically and compositionally distinct entities. Finally, by generating time-resolved photoemission sequences of the photo-excited carrier trapping process(10,11), we reveal a hole-trapping character with the kinetics limited by diffusion of holes to the local trap clusters. Our approach shows that managing structure and composition on the nanoscale will be essential for optimal performance of halide perovskite devices.


  
Capillary Trapping of CO2 in Sandstone Using Low Field NMR Relaxometry 期刊论文
WATER RESOURCES RESEARCH, 2019, 55 (12) : 10466-10478
作者:  Connolly, Paul R. J.;  Vogt, Sarah J.;  Mahmoud, Mohamed;  Ng, Christopher N. Y.;  May, Eric F.;  Johns, Michael L.
收藏  |  浏览/下载:20/0  |  提交时间:2020/02/16
Carbon sequestration  capillary trapping  NMR relaxation  
Capillary Trapping Following Imbibition in Porous Media: Microfluidic Quantification of the Impact of Pore-Scale Surface Roughness 期刊论文
WATER RESOURCES RESEARCH, 2019
作者:  Mehmani, Ayaz;  Kelly, Shaina;  Torres-Verdin, Carlos;  Balhoff, Matthew
收藏  |  浏览/下载:40/0  |  提交时间:2020/02/16
imbibition  capillary trapping  microfluidics  surface roughness  porous media  
Residual Trapping of CO2 in an Oil-Filled, Oil-Wet Sandstone Core: Results of Three-Phase Pore-Scale Imaging 期刊论文
GEOPHYSICAL RESEARCH LETTERS, 2019
作者:  Iglauer, Stefan;  Paluszny, Adriana;  Rahman, Taufiq;  Zhang, Yihuai;  Wulling, Wolfgang;  Lebedev, Maxim
收藏  |  浏览/下载:15/0  |  提交时间:2019/11/27
CO2-geosequestration  oil reservoir  pore-scale flow  residual trapping  three-phase flow  x-ray microtomography  
Temperature-Driven Bubble Migration as Proxy for Internal Bubble Pressures and Bubble Trapping Function in Ice Cores 期刊论文
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2019
作者:  Dadic, R.;  Schneebeli, M.;  Wiese, M.;  Bertler, N. A. N.;  Salamatin, A. N.;  Theile, T. C.;  Alley, R. B.;  Lipenkov, V. Ya.
收藏  |  浏览/下载:23/0  |  提交时间:2019/11/27
air bubbles  ice cores  pressure distribution  bubble trapping function  past changes  
Timber harvest jeopardize marten persistence in the heart of its range 期刊论文
FOREST ECOLOGY AND MANAGEMENT, 2019, 442: 46-52
作者:  Lavoie, Maxime;  Renard, Aurelie;  Lariviere, Serge
收藏  |  浏览/下载:11/0  |  提交时间:2019/11/26
Mattes Americana  Population dynamics  Conservation  Harvest  Trapping  Climate change  Logging  
Effect of rainfall on nocturnal activity of the Japanese dormouse 期刊论文
CLIMATE RESEARCH, 2019, 78 (3) : 205-209
作者:  Suzuki, Kei K.;  Ando, Motokazu
收藏  |  浏览/下载:10/0  |  提交时间:2019/11/26
Activity pattern  Precipitation  Climate change  Mammal  Camera trapping  
Topological Persistence for Relating Microstructure and Capillary Fluid Trapping in Sandstone 期刊论文
WATER RESOURCES RESEARCH, 2019, 55 (1) : 555-573
作者:  Herring, A. L.;  Robins, V;  Sheppard, A. P.
收藏  |  浏览/下载:30/0  |  提交时间:2019/04/09
capillary trapping  porous media  pore network  persistent homology  topology  multiphase flow