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DOI10.1038/nature23295
Evidence of high-temperature exciton condensation in two-dimensional atomic double layers
Wang, Zefang1; Rhodes, Daniel A.2; Watanabe, Kenji3; Taniguchi, Takashi3; Hone, James C.2; Shan, Jie1,4,5; Mak, Kin Fai1,4,5
2019-10-03
发表期刊NATURE
ISSN0028-0836
EISSN1476-4687
出版年2019
卷号574期号:7776页码:76-+
文章类型Article
语种英语
国家USA; Japan
英文摘要

A Bose-Einstein condensate is the ground state of a dilute gas of bosons, such as atoms cooled to temperatures close to absolute zero(1). With much smaller mass, excitons (bound electron-hole pairs) are expected to condense at considerably higher temperatures(2-7). Two-dimensional van der Waals semiconductors with very strong exciton binding are ideal systems for the study of high-temperature exciton condensation. Here we study electrically generated interlayer excitons in MoSe2-WSe2 atomic double layers with a density of up to 10(12) excitons per square centimetre. The interlayer tunnelling current depends only on the exciton density, which is indicative of correlated electron-hole pair tunnelling(8). Strong electroluminescence arises when a hole tunnels from WSe2 to recombine with an electron in MoSe2. We observe a critical threshold dependence of the electroluminescence intensity on exciton density, accompanied by super-Poissonian photon statistics near the threshold, and a large electroluminescence enhancement with a narrow peak at equal electron and hole densities. The phenomenon persists above 100 kelvin, which is consistent with the predicted critical condensation temperature(9-12). Our study provides evidence for interlayer exciton condensation in two-dimensional atomic double layers and opens up opportunities for exploring condensate-based optoelectronics and exciton-mediated high-temperature superconductivity(13).


领域地球科学 ; 气候变化 ; 资源环境
收录类别SCI-E
WOS记录号WOS:000488832500033
WOS关键词BOSE-EINSTEIN CONDENSATION ; TRANSITION ; COHERENCE ; PHASE
WOS类目Multidisciplinary Sciences
WOS研究方向Science & Technology - Other Topics
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文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/202794
专题地球科学
资源环境科学
气候变化
作者单位1.Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA;
2.Columbia Univ, Dept Mech Engn, New York, NY 10027 USA;
3.Natl Inst Mat Sci, Tsukuba, Ibaraki, Japan;
4.Cornell Univ, Lab Atom & Solid State Phys, Ithaca, NY 14850 USA;
5.Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA
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GB/T 7714
Wang, Zefang,Rhodes, Daniel A.,Watanabe, Kenji,et al. Evidence of high-temperature exciton condensation in two-dimensional atomic double layers[J]. NATURE,2019,574(7776):76-+.
APA Wang, Zefang.,Rhodes, Daniel A..,Watanabe, Kenji.,Taniguchi, Takashi.,Hone, James C..,...&Mak, Kin Fai.(2019).Evidence of high-temperature exciton condensation in two-dimensional atomic double layers.NATURE,574(7776),76-+.
MLA Wang, Zefang,et al."Evidence of high-temperature exciton condensation in two-dimensional atomic double layers".NATURE 574.7776(2019):76-+.
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