GSTDTAP  > 地球科学
DOI10.5194/acp-17-12779-2017
Do contemporary (1980-2015) emissions determine the elemental carbon deposition trend at Holtedahlfonna glacier, Svalbard?
Ruppel, Meri M.1; Soares, Joana2,3; Gallet, Jean-Charles4; Isaksson, Elisabeth4; Martma, Tonu5; Svensson, Jonas1,2; Kohler, Jack4; Pedersen, Christina A.4; Manninen, Sirkku1; Korhola, Atte1; Strom, Johan6
2017-10-26
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2017
卷号17期号:20
文章类型Article
语种英语
国家Finland; Canada; Norway; Estonia; Sweden
英文摘要

The climate impact of black carbon (BC) is notably amplified in the Arctic by its deposition, which causes albedo decrease and subsequent earlier snow and ice spring melt. To comprehensively assess the climate impact of BC in the Arctic, information on both atmospheric BC concentrations and deposition is essential. Currently, Arctic BC deposition data are very scarce, while atmospheric BC concentrations have been shown to generally decrease since the 1990s. However, a 300-year Svalbard ice core showed a distinct increase in EC (elemental carbon, proxy for BC) deposition from 1970 to 2004 contradicting atmospheric measurements and modelling studies. Here, our objective was to decipher whether this increase has continued in the 21st century and to investigate the drivers of the observed EC deposition trends. For this, a shallow firn core was collected from the same Svalbard glacier, and a regional-to-meso-scale chemical transport model (SILAM) was run from 1980 to 2015. The ice and firn core data indicate peaking EC deposition values at the end of the 1990s and lower values thereafter. The modelled BC deposition results generally support the observed glacier EC variations. However, the ice and firn core results clearly deviate from both measured and modelled atmospheric BC concentration trends, and the modelled BC deposition trend shows variations seemingly independent from BC emission or atmospheric BC concentration trends. wet-deposited at this Svalbard glacier, indicating that meteorological processes such as precipitation and scavenging efficiency have most likely a stronger influence on the BC deposition trend than BC emission or atmospheric concentration trends. BC emission source sectors contribute differently to the modelled atmospheric BC concentrations and BC deposition, which further supports our conclusion that different processes affect atmospheric BC concentration and deposition trends. Consequently, Arctic BC deposition trends should not directly be inferred based on atmospheric BC measurements, and more observational BC deposition data are required to assess the climate impact of BC in Arctic snow.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000413757200005
WOS关键词BIOMASS BURNING EMISSIONS ; VESTFONNA ICE CAP ; BLACK CARBON ; ASSIMILATION SYSTEM ; SNOW ; MODEL ; DISPERSION ; PARTICLES ; SPITSBERGEN ; VARIABILITY
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/22784
专题地球科学
作者单位1.Univ Helsinki, Dept Environm Sci, Helsinki 00790, Finland;
2.Finnish Meteorol Inst, Helsinki 00560, Finland;
3.Environm & Climate Change Canada, Air Qual Res Div, Toronto, ON M3H 5T4, Canada;
4.Norwegian Polar Res Inst, N-9296 Tromso, Norway;
5.Tallinn Univ Technol, Dept Geol, EE-19086 Tallinn, Estonia;
6.Stockholm Univ, Department Environm Sci & Analyt Chem, ACES Atmospher Sci Unit, S-11418 Stockholm, Sweden
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GB/T 7714
Ruppel, Meri M.,Soares, Joana,Gallet, Jean-Charles,et al. Do contemporary (1980-2015) emissions determine the elemental carbon deposition trend at Holtedahlfonna glacier, Svalbard?[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2017,17(20).
APA Ruppel, Meri M..,Soares, Joana.,Gallet, Jean-Charles.,Isaksson, Elisabeth.,Martma, Tonu.,...&Strom, Johan.(2017).Do contemporary (1980-2015) emissions determine the elemental carbon deposition trend at Holtedahlfonna glacier, Svalbard?.ATMOSPHERIC CHEMISTRY AND PHYSICS,17(20).
MLA Ruppel, Meri M.,et al."Do contemporary (1980-2015) emissions determine the elemental carbon deposition trend at Holtedahlfonna glacier, Svalbard?".ATMOSPHERIC CHEMISTRY AND PHYSICS 17.20(2017).
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