GSTDTAP  > 地球科学
DOI10.5194/acp-20-7217-2020
Heavy air pollution with a unique "non-stagnant" atmospheric boundary layer in the Yangtze River middle basin aggravated by regional transport of PM2.5 over China
Yu, Chao1,2; Zhao, Tianliang1; Bai, Yongqing3; Zhang, Lei1,4; Kong, Shaofei5; Yu, Xingna1; He, Jinhai1; Cui, Chunguang3; Yang, Jie1; You, Yingchang1; Ma, Guoxu1; Wu, Ming1; Chang, Jiacheng1
2020-06-23
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2020
卷号20期号:12页码:7217-7230
文章类型Article
语种英语
国家Peoples R China
英文摘要

The regional transport of air pollutants, controlled by emission sources and meteorological factors, results in a complex source-receptor relationship of air pollution change. Wuhan, a metropolis in the Yangtze River middle basin (YRMB) of central China, experienced heavy air pollution characterized by hourly PM2.5 concentrations reaching 471.1 mu g m(-3) in January 2016. To investigate the regional transport of PM2.5 over central eastern China (CEC) and the meteorological impact on wintertime air pollution in the YRMB area, observed meteorological and other relevant environmental data from January 2016 were analyzed. Our analysis presented noteworthy cases of heavy PM2.5 pollution in the YRMB area with unique "non-stagnant" meteorological conditions of strong northerly winds, no temperature inversion, and additional unstable structures in the atmospheric boundary layer. This unique set of conditions differed from the stagnant meteorological conditions characterized by near-surface weak winds, air temperature inversion, and stable structure in the boundary layer that are typically observed in heavy air pollution over most regions in China. The regional transport of PM2.5 over CEC aggravated PM2.5 levels, thus creating heavy air pollution in the YRMB area. This demonstrates a source-receptor relationship between the originating air pollution regions in CEC and the receiving YRMB region. Furthermore, a backward trajectory simulation using a Flexible Particle dispersion (FLEXPART) Weather Research and Forecasting (WRF) model to integrate the air pollutant emission inventory over China was used to explore the patterns of regional transport of PM2.5 governed by the strong northerly winds in the cold air activity of the East Asian winter monsoon season. It was estimated that the regional transport of PM2.5 from non-local air pollutant emissions contributes more than 65 % of the PM2.5 concentrations to the heavy air pollution in the YRMB region during the study period, revealing the importance of the regional transport of air pollutants over China as a causative factor of heavy air pollution over the YRMB area.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000543717500001
WOS关键词PARTICLE DISPERSION MODEL ; PARTICULATE MATTER ; METEOROLOGICAL CONDITIONS ; AEROSOL COMPOSITIONS ; EASTERN CHINA ; HAZE EVENTS ; VARIABILITY ; FLEXPART ; EMISSIONS ; CLIMATE
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
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被引频次:62[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/278088
专题地球科学
作者单位1.Nanjing Univ Informat Sci & Technol, Collaborat Innovat Ctr Forecast & Evaluat Meteoro, Key Lab Aerosol Cloud Precipitat, China Meteorol Adm,PREMIC, Nanjing 210044, Peoples R China;
2.China Power Engn Consulting Grp, Southwest Elect Power Design Inst Co Ltd, Chengdu 610021, Peoples R China;
3.China Meteorol Adm, Inst Heavy Rain, Wuhan 430205, Peoples R China;
4.Chengdu Acad Environm Sci, Chengdu 610031, Peoples R China;
5.China Univ Geosci Wuhan, Sch Environm Studies, Dept Atmospher Sci, Wuhan 430074, Peoples R China
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Yu, Chao,Zhao, Tianliang,Bai, Yongqing,et al. Heavy air pollution with a unique "non-stagnant" atmospheric boundary layer in the Yangtze River middle basin aggravated by regional transport of PM2.5 over China[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2020,20(12):7217-7230.
APA Yu, Chao.,Zhao, Tianliang.,Bai, Yongqing.,Zhang, Lei.,Kong, Shaofei.,...&Chang, Jiacheng.(2020).Heavy air pollution with a unique "non-stagnant" atmospheric boundary layer in the Yangtze River middle basin aggravated by regional transport of PM2.5 over China.ATMOSPHERIC CHEMISTRY AND PHYSICS,20(12),7217-7230.
MLA Yu, Chao,et al."Heavy air pollution with a unique "non-stagnant" atmospheric boundary layer in the Yangtze River middle basin aggravated by regional transport of PM2.5 over China".ATMOSPHERIC CHEMISTRY AND PHYSICS 20.12(2020):7217-7230.
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