GSTDTAP  > 地球科学
DOI10.1016/j.atmosres.2019.104833
PM2.5 in Abuja, Nigeria: Chemical characterization, source apportionment, temporal variations, transport pathways and the health risks assessment
Sulaymon, Ishaq Dimeji1,2; Mei, Xiaodong1,2; Yang, Shujian1,2; Chen, Sumin1,2; Zhang, Yang1,2; Hopke, Philip K.3,4; Schauer, James J.5,6; Zhang, Yuanxun1,2,7
2020-06-01
发表期刊ATMOSPHERIC RESEARCH
ISSN0169-8095
EISSN1873-2895
出版年2020
卷号237
文章类型Article
语种英语
国家Peoples R China; USA
英文摘要

Due to rapid industrial development and urbanization, Abuja is characterized with poor and deteriorated air quality. The level of PM(2.5 )concentrations in Abuja is very high and above the statutory limits; however, the high levels of pollution in Lugbe do not seem to be consistent with local emission sources. This study analyzed the chemical composition of PM2.5 to perform source identification and contributions in Lugbe, Abuja, Nigeria. Sampling in 2016 provided 246 PM2.5 samples at 2 sites across all the four months of sampling. The highest ambient PM2.5 concentration (142 pg m(-3)) was recorded in winter while the lowest (84 pg m -3 ) was observed in summer. Chemical mass closure suggested that dust (40.5%) contributed most of the PM2.5 mass. Source apportionment of PM2.5 was performed using positive matrix factorization (PMF) model and six sources were identified. They include mineral dust, crustal dust, vehicle exhaust, secondary nitrate, secondary sulfate, and industrial sources. Crustal dust, vehicle exhaust, and secondary sulfate were the major sources of ambient PM2.5 in Lugbe, contributing 33.3, 29.8, and 18.0%, respectively. The results of 120-h backward trajectories showed that external northeastern region was more dominant in January, while during the remaining three months, southwesterly winds prevailed. The results of bivariate polar plots for most of the factors showed the influence of the southern areas of Lugbe. The study found that there was long-range regional transport of PM2.5 into Lugbe area throughout the four months. Risk assessments revealed that ingestion route was the major exposure pathway for both children and adults. Non-carcinogenic and carcinogenic risk levels were below the acceptable threshold limits. Finally, the results of this study have shown that ambient air quality in Lugbe can be substantially improved by reducing the emissions from crustal dust, vehicle exhaust, and secondary sulfate sources in the external southern regions.


英文关键词Source apportionment Regional long-range transport PMF Heavy metals Health risks Abuja
领域地球科学
收录类别SCI-E
WOS记录号WOS:000525323100021
WOS关键词POSITIVE MATRIX FACTORIZATION ; BACKGROUND SITE ; POLAR PLOTS ; POLLUTION ; EMISSIONS ; EXPOSURES ; NITRATE ; METALS ; CHINA ; PM10
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
引用统计
被引频次:40[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/278905
专题地球科学
作者单位1.Univ Chinese Acad Sci, Coll Resources & Environm, Beijing 100049, Peoples R China;
2.Chinese Acad Sci, Huairou Ecoenvironm Observ, Beijing 101408, Peoples R China;
3.Clarkson Univ, Ctr Air Resources Engn & Sci, Potsdam, NY 13699 USA;
4.Univ Rochester, Dept Publ Hlth Sci, Sch Med & Dent, Rochester, NY 14642 USA;
5.Univ Wisconsin, Wisconsin State Lab Hyg, Madison, WI 53706 USA;
6.Univ Wisconsin, Environm Chem & Technol Program, Madison, WI 53705 USA;
7.Chinese Acad Sci, CAS Ctr Excellence Reg Atmospher Environm, Xiamen 361021, Peoples R China
推荐引用方式
GB/T 7714
Sulaymon, Ishaq Dimeji,Mei, Xiaodong,Yang, Shujian,et al. PM2.5 in Abuja, Nigeria: Chemical characterization, source apportionment, temporal variations, transport pathways and the health risks assessment[J]. ATMOSPHERIC RESEARCH,2020,237.
APA Sulaymon, Ishaq Dimeji.,Mei, Xiaodong.,Yang, Shujian.,Chen, Sumin.,Zhang, Yang.,...&Zhang, Yuanxun.(2020).PM2.5 in Abuja, Nigeria: Chemical characterization, source apportionment, temporal variations, transport pathways and the health risks assessment.ATMOSPHERIC RESEARCH,237.
MLA Sulaymon, Ishaq Dimeji,et al."PM2.5 in Abuja, Nigeria: Chemical characterization, source apportionment, temporal variations, transport pathways and the health risks assessment".ATMOSPHERIC RESEARCH 237(2020).
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