GSTDTAP  > 气候变化
DOI10.1029/2019JD031535
Individual Particle Characteristics, Optical Properties and Evolution of an Extreme Long-Range Transported Biomass Burning Event in the European Arctic (Ny-angstrom lesund, Svalbard Islands)
Moroni, B.1; Ritter, C.2; Crocchianti, S.1; Markowicz, K.3; Mazzola, M.4; Becagli, S.4,5; Traversi, R.4,5; Krejci, R.6; Tunved, P.6; Cappelletti, D.1
2020-03-16
发表期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
EISSN2169-8996
出版年2020
卷号125期号:5
文章类型Article
语种英语
国家Italy; Germany; Poland; Sweden
英文摘要

This paper reports an exceptional biomass burning (BB) advection event from Alaska registered at Ny-angstrom lesund from 10 to 17 July 2015 with particular interest on the influence of the airborne particle characteristics on the optical properties of the aerosol during the event. To this purpose we considered two DEKATI 12-stage aerosol samples spanning the entire advection and analyzed them by scanning electron microscopy techniques. Aerosol chemical data and microphysical properties were also evaluated in order to correlate any change of individual particle characteristics with the bulk properties of the aerosol. The results of individual particle analysis depict a complex event characterized by a first phase (P1) of massive input of BB carbonaceous particles (i.e., tar balls, popcorn refractory particles, and organic particles), and by a second phase (P2) dominated by inorganic salts. The peculiar feature of this BB event is the exceptionally large grain size of the subspherical organic particles at the beginning of the event with respect to the background. At these conditions a significant increase of the scattering efficiency may occur even for a small increase of the size parameter. Results of the simulation of the complex refractive indices (n-ik) confirm this evaluation. Aerosol evolution during the event resulted from the combination of three distinct occurrences: (a) progressive rotation of air mass circulation toward non-BB source areas, (b) development of a thick fog layer in the planetary boundary layer, and (c) sea salt spray direct advection of local/regional provenance.


英文关键词SEM-EDS particle size distribution aerosol optical properties closure studies aerosol evolution
领域气候变化
收录类别SCI-E
WOS记录号WOS:000519602000015
WOS关键词ATMOSPHERIC TAR BALLS ; BROWN CARBON ; BLACK CARBON ; AEROSOL-PARTICLES ; ABSORPTION PROPERTIES ; REFRACTIVE-INDEX ; SOUTHERN AFRICA ; ORGANIC-ACIDS ; CAVITY RING ; EMISSIONS
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/280099
专题气候变化
作者单位1.Univ Perugia, Dept Chem Biol & Biotechnol, Perugia, Italy;
2.Alfred Wegener Inst, Helmoltz Ctr Polar & Marine Res, Potsdam, Germany;
3.Univ Warsaw, Fac Phys, Inst Geophys, Warsaw, Poland;
4.Natl Res Council Italy, Inst Polar Sci, Bologna, Italy;
5.Univ Florence, Dept Chem, Sesto Fiorentino, Italy;
6.Stockholm Univ, Dept Environm Sci & Analyt Chem ACES, Stockholm, Sweden
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GB/T 7714
Moroni, B.,Ritter, C.,Crocchianti, S.,et al. Individual Particle Characteristics, Optical Properties and Evolution of an Extreme Long-Range Transported Biomass Burning Event in the European Arctic (Ny-angstrom lesund, Svalbard Islands)[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2020,125(5).
APA Moroni, B..,Ritter, C..,Crocchianti, S..,Markowicz, K..,Mazzola, M..,...&Cappelletti, D..(2020).Individual Particle Characteristics, Optical Properties and Evolution of an Extreme Long-Range Transported Biomass Burning Event in the European Arctic (Ny-angstrom lesund, Svalbard Islands).JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,125(5).
MLA Moroni, B.,et al."Individual Particle Characteristics, Optical Properties and Evolution of an Extreme Long-Range Transported Biomass Burning Event in the European Arctic (Ny-angstrom lesund, Svalbard Islands)".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 125.5(2020).
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