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DOI10.1029/2019JD031827
Temporal Characteristics and Potential Sources of Black Carbon in Megacity Shanghai, China
Wei, C.1,2; Wang, M. H.1,2; Fu, Q. Y.3; Dai, C.1,2; Huang, R.3; Bao, Q.3
2020-05-16
发表期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
EISSN2169-8996
出版年2020
卷号125期号:9
文章类型Article
语种英语
国家Peoples R China
英文摘要

Black carbon (BC) is a major light absorption material that acts as a climate change driver with high radiative forcing and as an air pollutant that reduces visibility and air quality. Thus, reducing the emission and ambient concentration of BC could help address climate change and improve air quality simultaneously. In this study, the mass concentration of atmospheric BC was continuously measured by an aethalometer in Shanghai in 2017. The annual BC concentration was 2.19 +/- 1.28 mu g/m(3), with the highest loading in winter and the lowest loading in autumn. The BC concentrations varied with year and location when compared with previous studies in different locations in Shanghai. The hourly BC concentration had a bimodal distribution, with two peaks during the morning and evening traffic rush hours. Liquid fuels, biomass, and coal combustion contributed 65.7%, 21.5%, and 12.8%, respectively, of the total BC based on the advanced aethalometer model. The three sources varied in different seasons with a high contribution of liquid source in summer and more coal and biomass emissions in winter. High BC concentrations accumulated in the stable weather conditions in the four seasons and appeared when there were high wind speeds from the northwestern direction in winter. The Yangtze River Delta region was the most likely potential source region of high BC loading in the four seasons, and long-range transport from North China in winter was another likely source region based on the results of cluster analysis and potential source contribution function analysis of backward trajectories.


英文关键词black carbon temporal variation source apportionment meteorological condition back trajectory
领域气候变化
收录类别SCI-E
WOS记录号WOS:000536605500006
WOS关键词POLYCYCLIC AROMATIC-HYDROCARBONS ; FINE PARTICULATE MATTER ; SOURCE APPORTIONMENT ; AEROSOL ; EMISSIONS ; POLLUTION ; WINTER ; XIAN ; DERIVATIVES ; EPISODES
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
引用统计
被引频次:36[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/280209
专题气候变化
作者单位1.Chinese Acad Sci, Shanghai Carbon Data Res Ctr, Shanghai Adv Res Inst, Shanghai, Peoples R China;
2.Chinese Acad Sci, Shanghai Adv Res Inst, CAS Key Lab Low Carbon Convers Sci & Engn, Shanghai, Peoples R China;
3.Shanghai Environm Monitoring Ctr, Shanghai, Peoples R China
推荐引用方式
GB/T 7714
Wei, C.,Wang, M. H.,Fu, Q. Y.,et al. Temporal Characteristics and Potential Sources of Black Carbon in Megacity Shanghai, China[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2020,125(9).
APA Wei, C.,Wang, M. H.,Fu, Q. Y.,Dai, C.,Huang, R.,&Bao, Q..(2020).Temporal Characteristics and Potential Sources of Black Carbon in Megacity Shanghai, China.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,125(9).
MLA Wei, C.,et al."Temporal Characteristics and Potential Sources of Black Carbon in Megacity Shanghai, China".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 125.9(2020).
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