GSTDTAP  > 气候变化
DOI10.1029/2019JD031961
Mobile Laboratory Measurements of High Surface Ozone Levels and Spatial Heterogeneity During LISTOS 2018: Evidence for Sea Breeze Influence
Zhang, Jie1; Ninneman, Matthew1; Joseph, Everette1,2; Schwab, Margaret J.1; Shrestha, Bhupal1; Schwab, James J.1
2020-06-16
发表期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
EISSN2169-8996
出版年2020
卷号125期号:11
文章类型Article
语种英语
国家USA
英文摘要

The Long Island Sound Tropospheric Ozone Study (LISTOS) was organized to investigate ozone formation and transport in the New York City metropolitan area and locations downwind. During LISTOS, the University at Albany Atmospheric Sciences Research Center (ASRC) mobile laboratory was used for measuring surface O-3, NO2, and aerosol number and mass concentration. Sharp O-3 concentration gradients, with Delta O-3 Delta y(-1) over 15 ppb km(-1), were measured both at and near the land-water interface and on the highway on days characterized by high regional O-3 concentrations. These large O-3 gradients at or near the land-water interface, and in air masses relatively low in NO2, are shown to be influenced in part by the transport of highly oxidized air masses via sea breeze circulation and convergence with gradient flow. On the highway under regionally high O-3 concentrations, strong anticorrelation (R-2 = 0.78, p < 0.05) between O-3 and NO2 and an absolute slope less than 1 suggested that O-x concentrations (O-3 + NO2) increased with increasing NO2. Overall, the on-road measurements made during LISTOS help to better characterize the interaction between the emitted pollution and the meteorological conditions on Long Island, thereby having potential policy implications.


Plain Language Summary Ozone pollution is a significant problem for the New York City (NYC) Metropolitan Area, which has been classified by the U.S. Environmental Protection Agency as being in noncompliance with the National Ambient Air Quality Standard for ozone. The southern coast of Connecticut is the most severely affected by ozone pollution, which is produced in the atmosphere as it travels downwind from emission sources of precursor gases like oxides of nitrogen and volatile organic compounds. The impact of ozone on a given location involves a complex interplay of emissions, meteorology, and chemistry. Our study explored aspects of this interplay on several polluted days in summer 2018 using a Dodge Sprinter van mobile laboratory equipped with instrumentation to measure ozone, one of the critical oxides of nitrogen, and other parameters. Some of the analysis days yielded significant and rapid changes in ozone concentration near the south or north shore of Long Island. Our results suggest that sea breeze winds can greatly influence ozone concentrations near the coast in some cases. Understanding when and how the sea breeze affects air quality in regions downwind of NYC and other coastal metropolitan areas will help efforts to improve air quality in these locations.


英文关键词LISTOS sea breeze ozone gradients on-road measurements
领域气候变化
收录类别SCI-E
WOS记录号WOS:000541156800008
WOS关键词AEROSOL MASS-SPECTROMETER ; NEW-YORK-CITY ; HIGH-RESOLUTION ; LAKE BREEZES ; BAY-BREEZE ; AIR-QUALITY ; IMPACT ; CIRCULATIONS ; SUMMER ; OXIDES
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/289459
专题气候变化
作者单位1.SUNY Albany, Atmospher Sci Res Ctr, Albany, NY 12222 USA;
2.Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA
推荐引用方式
GB/T 7714
Zhang, Jie,Ninneman, Matthew,Joseph, Everette,et al. Mobile Laboratory Measurements of High Surface Ozone Levels and Spatial Heterogeneity During LISTOS 2018: Evidence for Sea Breeze Influence[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2020,125(11).
APA Zhang, Jie,Ninneman, Matthew,Joseph, Everette,Schwab, Margaret J.,Shrestha, Bhupal,&Schwab, James J..(2020).Mobile Laboratory Measurements of High Surface Ozone Levels and Spatial Heterogeneity During LISTOS 2018: Evidence for Sea Breeze Influence.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,125(11).
MLA Zhang, Jie,et al."Mobile Laboratory Measurements of High Surface Ozone Levels and Spatial Heterogeneity During LISTOS 2018: Evidence for Sea Breeze Influence".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 125.11(2020).
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