GSTDTAP  > 地球科学
DOI10.5194/acp-18-12953-2018
Intermittent turbulence contributes to vertical dispersion of PM2.5 in the North China Plain: cases from Tianjin
Wei, Wei1; Zhang, Hongsheng2; Wu, Bingui3; Huang, Yongxiang4; Cai, Xuhui5; Song, Yu5; Li, Jianduo1
2018-09-10
发表期刊ATMOSPHERIC CHEMISTRY AND PHYSICS
ISSN1680-7316
EISSN1680-7324
出版年2018
卷号18期号:17页码:12953-12967
文章类型Article
语种英语
国家Peoples R China
英文摘要

Heavy particulate pollution events have frequently occurred in the North China Plain over the past decades. Due to high emissions and poor dispersion conditions, issues are becoming increasingly serious during cold seasons. Although early studies have explored some potential reasons for air pollution, there are few works focusing on the effects of intermittent turbulence. This paper draws upon two typical PM2.5 (particulate matter with diameter less than 2.5 mm) pollution cases from the winter of 2016-2017. After several days of gradual accumulation, the concentration of PM2.5 near the surface reached the maximum as a combined result of strong inversion layer, stagnant wind, and high ambient humidity and then sharply decreased to a very low level within a few hours. In order to identify the strength of turbulent intermittency, an effective index, called the intermittency factor (IF), was proposed by this work. The results show that the turbulence is very weak during the cumulative stage due to the suppression by strongly stratified layers, while for the stage of dispersion, the turbulence is highly intermittent and not locally generated. The vertical structure of turbulence and wind profiles confirms the generation and downward transport of intermittent turbulence associated with low-level jets. The intermittent turbulent fluxes contribute positively to the vertical transport of particulate matter and improve the air quality near the surface. This work has demonstrated a possible mechanism of how intermittent turbulence affects the dispersion of particulate matter.


领域地球科学
收录类别SCI-E
WOS记录号WOS:000444187300001
WOS关键词STABLE BOUNDARY-LAYER ; HETEROGENEOUS AQUEOUS REACTIONS ; EMPIRICAL MODE DECOMPOSITION ; PARTICULATE MATTER PM2.5 ; LOW-LEVEL JET ; AIR-POLLUTION ; SECONDARY FORMATION ; REGIONAL TRANSPORT ; INORGANIC AEROSOLS ; HEBEI REGION
WOS类目Environmental Sciences ; Meteorology & Atmospheric Sciences
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/31084
专题地球科学
作者单位1.Chinese Acad Meteorol Sci, State Key Lab Severe Weather, Beijing 100081, Peoples R China;
2.Peking Univ, Sch Phys, Dept Atmospher & Ocean Sci, Lab Climate & Ocean Atmosphere Studies, Beijing 100081, Peoples R China;
3.Tianjin Municipal Meteorol Bur, Tianjin 300074, Peoples R China;
4.Xiamen Univ, State Key Lab Marine Environm Sci, Xiamen 361005, Peoples R China;
5.Peking Univ, Dept Environm Sci, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100081, Peoples R China
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GB/T 7714
Wei, Wei,Zhang, Hongsheng,Wu, Bingui,et al. Intermittent turbulence contributes to vertical dispersion of PM2.5 in the North China Plain: cases from Tianjin[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2018,18(17):12953-12967.
APA Wei, Wei.,Zhang, Hongsheng.,Wu, Bingui.,Huang, Yongxiang.,Cai, Xuhui.,...&Li, Jianduo.(2018).Intermittent turbulence contributes to vertical dispersion of PM2.5 in the North China Plain: cases from Tianjin.ATMOSPHERIC CHEMISTRY AND PHYSICS,18(17),12953-12967.
MLA Wei, Wei,et al."Intermittent turbulence contributes to vertical dispersion of PM2.5 in the North China Plain: cases from Tianjin".ATMOSPHERIC CHEMISTRY AND PHYSICS 18.17(2018):12953-12967.
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