资源环境科技发展态势分析平台

Arctic observations show large decreases in the concentrations of sulfate and black carbon (BC) aerosols since the early 1980s. These near-term climate-forcing pollutants perturb the radiative balance of the atmosphere and may have played an important role in recent Arctic warming. We use the GEOS-Chem global chemical transport model to construct a 3-D representation of Arctic aerosols that is generally consistent with observations and their trends from 1980 to 2010. Observations at Arctic surface sites show significant decreases in sulfate and BC mass concentrations of 2-3% per year. We find that anthropogenic aerosols yield a negative forcing over the Arctic, with an average 2005-2010 Arctic shortwave radiative forcing (RF) of -0.190.05Wm(-2) at the top of atmosphere (TOA). Anthropogenic sulfate in our study yields more strongly negative forcings over the Arctic troposphere in spring (-1.170.10Wm(-2)) than previously reported. From 1980 to 2010, TOA negative RF by Arctic aerosol declined, from -0.670.06Wm(-2) to -0.190.05Wm(-2), yielding a net TOA RF of +0.48 +/- 0.06Wm(-2). The net positive RF is due almost entirely to decreases in anthropogenic sulfate loading over the Arctic. We estimate that 1980-2010 trends in aerosol-radiation interactions over the Arctic and Northern Hemisphere midlatitudes have contributed a net warming at the Arctic surface of +0.27 +/- 0.04K, roughly one quarter of the observed warming. Our study does not consider BC emissions from gas flaring nor the regional climate response to aerosol-cloud interactions or BC deposition on snow.