GSTDTAP  > 气候变化
DOI10.1002/2017JD027257
Using Observations and Source-Specific Model Tracers to Characterize Pollutant Transport During FRAPPE and DISCOVER-AQ
Pfister, G. G.1; Reddy, P. J.1,2; Barth, M. C.1; Flocke, F. F.1; Fried, A.3; Herndon, S. C.4; Sive, B. C.5; Sullivan, J. T.6; Thompson, A. M.6; Yacovitch, T. I.4; Weinheimer, A. J.1; Wisthaler, A.7
2017-10-16
发表期刊JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES
ISSN2169-897X
EISSN2169-8996
出版年2017
卷号122期号:19
文章类型Article
语种英语
国家USA; Norway
英文摘要

sport is a key parameter in air quality research and plays a dominant role in the Colorado Northern Front Range Metropolitan Area (NFRMA), where terrain-induced flows and recirculation patterns can lead to vigorous mixing of different emission sources. To assess different transport processes and their connection to air quality in the NFRMA during the FRAPP a DISCOVER-A Q campaigns in summer 2014, we use the Weather Research and Forecasting Model with inert tracers. Overall, the model represents well the measured winds, and the inert tracers are in good agreement with observations of comparable trace gas concentrations. The model tracers support the analysis of surface wind and ozone measurements and allow for the analysis of transport patterns and interactions of emissions. A main focus of this study is on characterizing pollution transport from the NFRMA to the mountains by mountain-valley flows and the potential for recirculating pollution back into the NFRMA. One such event on 12 August 2014 was well captured by the aircraft and is studied in more detail. The model represents the flow conditions and demonstrates that during upslope events, frequently, there is a separation of air masses that are heavily influenced by oil and gas emissions to the north and dominated by urban emissions to the south. This case study provides evidence that NFRMA pollution not only can impact the nearby foothills and mountain areas to the east of the Continental Divide but that pollution can "spillover" into the valleys to the west of the Continental Divide.


领域气候变化
收录类别SCI-E
WOS记录号WOS:000413675900021
WOS关键词COLORADO FRONT RANGE ; OH PHOTOCHEMISTRY EXPERIMENT ; MOUNTAIN NATIONAL-PARK ; ELEVATION GRADIENT ; UPPER TROPOSPHERE ; SURFACE OZONE ; AIR-QUALITY ; PARAMETERIZATION ; DISTRIBUTIONS ; ENTRAINMENT
WOS类目Meteorology & Atmospheric Sciences
WOS研究方向Meteorology & Atmospheric Sciences
引用统计
文献类型期刊论文
条目标识符http://119.78.100.173/C666/handle/2XK7JSWQ/33104
专题气候变化
作者单位1.Natl Ctr Atmospher Res, Atmospher Chem Observat & Modeling, POB 3000, Boulder, CO 80307 USA;
2.Colorado Dept Publ Hlth & Environm, Air Pollut Control Div, Boulder, CO USA;
3.Univ Colorado, Inst Arctic & Alpine Res, Boulder, CO 80309 USA;
4.Aerodyne Res Inc, Billerica, MA USA;
5.Natl Pk Serv, Air Resources Div, Denver, CO USA;
6.NASA, Goddard Space Flight Ctr, Earth Sci Div, Greenbelt, MD USA;
7.Univ Oslo, Dept Chem, Oslo, Norway
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Pfister, G. G.,Reddy, P. J.,Barth, M. C.,et al. Using Observations and Source-Specific Model Tracers to Characterize Pollutant Transport During FRAPPE and DISCOVER-AQ[J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,2017,122(19).
APA Pfister, G. G..,Reddy, P. J..,Barth, M. C..,Flocke, F. F..,Fried, A..,...&Wisthaler, A..(2017).Using Observations and Source-Specific Model Tracers to Characterize Pollutant Transport During FRAPPE and DISCOVER-AQ.JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES,122(19).
MLA Pfister, G. G.,et al."Using Observations and Source-Specific Model Tracers to Characterize Pollutant Transport During FRAPPE and DISCOVER-AQ".JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES 122.19(2017).
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