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Potential for large-scale CO2 removal via enhanced rock weathering with croplands 期刊论文
NATURE, 2020, 583 (7815) : 242-+
作者:  David J. Beerling;  Euripides P. Kantzas;  Mark R. Lomas;  Peter Wade;  Rafael M. Eufrasio;  Phil Renforth;  Binoy Sarkar;  M. Grace Andrews;  Rachael H. James;  Christopher R. Pearce;  Jean-Francois Mercure;  Hector Pollitt;  Philip B. Holden;  Neil R. Edwards;  Madhu Khanna;  Lenny Koh;  Shaun Quegan;  Nick F. Pidgeon;  Ivan A. Janssens;  James Hansen;  Steven A. Banwart
收藏  |  浏览/下载:18/0  |  提交时间:2020/07/14

Enhanced silicate rock weathering (ERW), deployable with croplands, has potential use for atmospheric carbon dioxide (CO2) removal (CDR), which is now necessary to mitigate anthropogenic climate change(1). ERW also has possible co-benefits for improved food and soil security, and reduced ocean acidification(2-4). Here we use an integrated performance modelling approach to make an initial techno-economic assessment for 2050, quantifying how CDR potential and costs vary among nations in relation to business-as-usual energy policies and policies consistent with limiting future warming to 2 degrees Celsius(5). China, India, the USA and Brazil have great potential to help achieve average global CDR goals of 0.5 to 2gigatonnes of carbon dioxide (CO2) per year with extraction costs of approximately US$80-180 per tonne of CO2. These goals and costs are robust, regardless of future energy policies. Deployment within existing croplands offers opportunities to align agriculture and climate policy. However, success will depend upon overcoming political and social inertia to develop regulatory and incentive frameworks. We discuss the challenges and opportunities of ERW deployment, including the potential for excess industrial silicate materials (basalt mine overburden, concrete, and iron and steel slag) to obviate the need for new mining, as well as uncertainties in soil weathering rates and land-ocean transfer of weathered products.


  
Effects of atmospheric circulations on the interannual variation in PM2.5 concentrations over the Beijing-Tianjin-Hebei region in 2013-2018 期刊论文
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2020, 20 (13) : 7667-7682
作者:  Wang, Xiaoyan;  Zhang, Renhe
收藏  |  浏览/下载:10/0  |  提交时间:2020/07/06
Modelling the potential impacts of the recent, unexpected increase in CFC-11 emissions on total column ozone recovery 期刊论文
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2020, 20 (12) : 7153-7166
作者:  Keeble, James;  Abraham, N. Luke;  Archibald, Alexander T.;  Chipperfield, Martyn P.;  Dhomse, Sandip;  Griffiths, Paul T.;  Pyle, John A.
收藏  |  浏览/下载:11/0  |  提交时间:2020/06/22
Dynamic projection of anthropogenic emissions in China: methodology and 2015-2050 emission pathways under a range of socio-economic, climate policy, and pollution control scenarios 期刊论文
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2020, 20 (9) : 5729-5757
作者:  Tong, Dan;  Cheng, Jing;  Liu, Yang;  Yu, Sha;  Yan, Liu;  Hong, Chaopeng;  Qin, Yu;  Zhao, Hongyan;  Zheng, Yixuan;  Geng, Guannan;  Li, Meng;  Liu, Fei;  Zhang, Yuxuan;  Zheng, Bo;  Clarke, Leon;  Zhang, Qiang
收藏  |  浏览/下载:24/0  |  提交时间:2020/08/18
Dynamic projection of anthropogenic emissions in China: methodology and 2015-2050 emission pathways under a range of socio-economic, climate policy, and pollution control scenarios 期刊论文
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2020, 20 (9) : 5729-5757
作者:  Tong, Dan;  Cheng, Jing;  Liu, Yang;  Yu, Sha;  Yan, Liu;  Hong, Chaopeng;  Qin, Yu;  Zhao, Hongyan;  Zheng, Yixuan;  Geng, Guannan;  Li, Meng;  Liu, Fei;  Zhang, Yuxuan;  Zheng, Bo;  Clarke, Leon;  Zhang, Qiang
收藏  |  浏览/下载:20/0  |  提交时间:2020/05/20
Effects of black carbon mitigation on Arctic climate 期刊论文
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2020, 20 (9) : 5527-5546
作者:  Kuhn, Thomas;  Kupiainen, Kaarle;  Miinalainen, Tuuli;  Kokkola, Harri;  Paunu, Ville-Veikko;  Laakso, Anton;  Tonttila, Juha;  Van Dingenen, Rita;  Kulovesi, Kati;  Karvosenoja, Niko;  Lehtinen, Kari E. J.
收藏  |  浏览/下载:14/0  |  提交时间:2020/05/13
Targeting of temperate phages drives loss of type I CRISPR-Cas systems 期刊论文
NATURE, 2020, 578 (7793) : 149-+
作者:  Xiang, Lifeng;  Yin, Yu;  Zheng, Yun;  Ma, Yanping;  Li, Yonggang;  Zhao, Zhigang;  Guo, Junqiang;  Ai, Zongyong;  Niu, Yuyu;  Duan, Kui;  He, Jingjing;  Ren, Shuchao;  Wu, Dan;  Bai, Yun;  Shang, Zhouchun;  Dai, Xi;  Ji, Weizhi;  Li, Tianqing
收藏  |  浏览/下载:31/0  |  提交时间:2020/07/03

On infection of their host, temperate viruses that infect bacteria (bacteriophages  hereafter referred to as phages) enter either a lytic or a lysogenic cycle. The former results in lysis of bacterial cells and phage release (resulting in horizontal transmission), whereas lysogeny is characterized by the integration of the phage into the host genome, and dormancy (resulting in vertical transmission)(1). Previous co-culture experiments using bacteria and mutants of temperate phages that are locked in the lytic cycle have shown that CRISPR-Cas systems can efficiently eliminate the invading phages(2,3). Here we show that, when challenged with wild-type temperate phages (which can become lysogenic), type I CRISPR-Cas immune systems cannot eliminate the phages from the bacterial population. Furthermore, our data suggest that, in this context, CRISPR-Cas immune systems are maladaptive to the host, owing to the severe immunopathological effects that are brought about by imperfect matching of spacers to the integrated phage sequences (prophages). These fitness costs drive the loss of CRISPR-Cas from bacterial populations, unless the phage carries anti-CRISPR (acr) genes that suppress the immune system of the host. Using bioinformatics, we show that this imperfect targeting is likely to occur frequently in nature. These findings help to explain the patchy distribution of CRISPR-Cas immune systems within and between bacterial species, and highlight the strong selective benefits of phage-encoded acr genes for both the phage and the host under these circumstances.


CRISPR-Cas systems cannot eliminate temperate bacteriophages from bacterial populations and-in this context-the systems impose immunopathological costs on the host, creating selective pressures that may explain their patchy distribution in bacteria.


  
Impact of air pollution control measures and regional transport on carbonaceous aerosols in fine particulate matter in urban Beijing, China: insights gained from long-term measurement 期刊论文
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2019, 19 (13) : 8569-8590
作者:  Ji, Dongsheng;  Gao, Wenkang;  Maenhaut, Willy;  He, Jun;  Wang, Zhe;  Li, Jiwei;  Du, Wupeng;  Wang, Lili;  Sun, Yang;  Xin, Jinyuan;  Hu, Bo;  Wang, Yuesi
收藏  |  浏览/下载:7/0  |  提交时间:2019/11/27
Simultaneous shipborne measurements of CO2, CH4 and CO and their application to improving greenhouse-gas flux estimates in Australia 期刊论文
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2019, 19 (10) : 7055-7072
作者:  Bukosa, Beata;  Deutscher, Nicholas M.;  Fisher, Jenny A.;  Kubistin, Dagmar;  Paton-Walsh, Clare;  Griffith, David W. T.
收藏  |  浏览/下载:6/0  |  提交时间:2019/11/26
Effects of air pollution control policies on PM2.5 pollution improvement in China from 2005 to 2017: a satellite-based perspective 期刊论文
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2019, 19 (10) : 6861-6877
作者:  Ma, Zongwei;  Liu, Riyang;  Liu, Yang;  Bi, Jun
收藏  |  浏览/下载:7/0  |  提交时间:2019/11/26