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Analysis of the Thermodynamic Phase Transition of Tracked Convective Clouds Based on Geostationary Satellite Observations 期刊论文
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2020, 125 (11)
作者:  Coopman, Q.;  Hoose, C.;  Stengel, M.
收藏  |  浏览/下载:21/0  |  提交时间:2020/08/18
Clouds  Glaciation temperature  geostationary satellite  SEVIRI  Thermodynamic phase  
Observations of grain-boundary phase transformations in an elemental metal 期刊论文
NATURE, 2020, 579 (7799) : 375-+
作者:  Valente, Luis;  Phillimore, Albert B.;  Melo, Martim;  Warren, Ben H.;  Clegg, Sonya M.;  Havenstein, Katja;  Tiedemann, Ralph;  Illera, Juan Carlos;  Thebaud, Christophe;  Aschenbach, Tina;  Etienne, Rampal S.
收藏  |  浏览/下载:29/0  |  提交时间:2020/07/03

Atomic-resolution observations combined with simulations show that grain boundaries within elemental copper undergo temperature-induced solid-state phase transformation to different structures  grain boundary phases can also coexist and are kinetically trapped structures.


The theory of grain boundary (the interface between crystallites, GB) structure has a long history(1) and the concept of GBs undergoing phase transformations was proposed 50 years ago(2,3). The underlying assumption was that multiple stable and metastable states exist for different GB orientations(4-6). The terminology '  complexion'  was recently proposed to distinguish between interfacial states that differ in any equilibrium thermodynamic property(7). Different types of complexion and transitions between complexions have been characterized, mostly in binary or multicomponent systems(8-19). Simulations have provided insight into the phase behaviour of interfaces and shown that GB transitions can occur in many material systems(20-24). However, the direct experimental observation and transformation kinetics of GBs in an elemental metal have remained elusive. Here we demonstrate atomic-scale GB phase coexistence and transformations at symmetric and asymmetric [111 over bar ] tilt GBs in elemental copper. Atomic-resolution imaging reveals the coexistence of two different structures at sigma 19b GBs (where sigma 19 is the density of coincident sites and b is a GB variant), in agreement with evolutionary GB structure search and clustering analysis(21,25,26). We also use finite-temperature molecular dynamics simulations to explore the coexistence and transformation kinetics of these GB phases. Our results demonstrate how GB phases can be kinetically trapped, enabling atomic-scale room-temperature observations. Our work paves the way for atomic-scale in situ studies of metallic GB phase transformations, which were previously detected only indirectly(9,15,27-29), through their influence on abnormal grain growth, non-Arrhenius-type diffusion or liquid metal embrittlement.


  
Influence of Wind Direction on Thermodynamic Properties and Arctic Mixed-Phase Clouds in Autumn at Utqiagvik, Alaska 期刊论文
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2018, 123 (17) : 9589-9603
作者:  Qiu, Shaoyue;  Xi, Baike;  Dong, Xiquan
收藏  |  浏览/下载:15/0  |  提交时间:2019/04/09
Arctic mixed-phase cloud  thermodynamic profile  wind direction  cloud occurrence frequency  cloud microphysical processes  cloud vertical structure  
Evaluation of wintertime precipitation forecasts over the Australian Snowy Mountains 期刊论文
ATMOSPHERIC RESEARCH, 2018, 207: 42-61
作者:  Huang, Yi;  Chubb, Thomas;  Sarmadi, Fahimeh;  Siems, Steven T.;  Manton, Michael J.;  Franklin, Charmaine N.;  Ebert, Elizabeth
收藏  |  浏览/下载:17/0  |  提交时间:2019/04/09
Orographic precipitation  Quantitative precipitation forecast  Australian Snowy Mountains  Synoptic regimes  Lower-atmosphere stability  Cloud thermodynamic phase  
Characterizing the information content of cloud thermodynamic phase retrievals from the notional PACE OCI shortwave reflectance measurements 期刊论文
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2017, 122 (15)
作者:  Coddington, O. M.;  Vukicevic, T.;  Schmidt, K. S.;  Platnick, S.
收藏  |  浏览/下载:8/0  |  提交时间:2019/04/09
cloud thermodynamic phase  shortwave radiation  passive remote sensing